We show that many-body correlations among excitons originating from the Pauli exclusion principle in a quantum well embedded inside a microcavity provide a possibility to produce pairs of entangled photons by ultrashort laser pulses with a yield of $\sim 10^{-2}$. The quantum-field theoretical two-particle density matrix in second quantization is used to calculate entanglement for arbitrary emission angles. %At time scales where the heavy-light hole splitting is resolved the resonances corresponding to different two-exciton %states develop, which allow for a simple kinematic theory relating the %states of the outgoing photons with the respective two-exciton states. Largest response can be expected at symmetric emission angles for resonances with the heavy-heavy and light-light two-exciton states with remarkably nontrivial dependence of entanglement on the emission angles and on the ellipticity parameters of the excitation. We show that the angle dependence can be tailored by means of the microcavity. Interestingly, the emitted entangled 2-photon states are always in a triplet state.
We show how a Dzyaloshinskii-Moriya interaction can be generated in an ultrathin metal film from the induced internal electric field created by an ultrashort electromagnetic pulse. This interaction does not require structural inversion-symmetry breaking, and its amplitude can be tuned depending on the amplitude of the field. We perform first-principles calculations to estimate the strength of the field-induced magnetoelectric coupling for ferromagnetic Fe, Co, and Ni, and antiferromagnetic Mn, as well as FePt alloys. Last, using atomistic simulations, we demonstrate how an isolated antiferroma…
We study the emission of femtosecond spin current pulses at Fe/Au interfaces. Using optical second harmonic generation we demonstrate the control of pulse shape and duration by varying the emitter thickness and show that it is determined by the parameters of hot electrons emission and the diffusive transport. Using a simple model of electron emission we develop a description of superdiffusive spin transport in Au allowing to extract electron velocity and scattering rates from the experimental data. The importance of carrier multiplication in Fe is demonstrated.
Recent advances in ultrashort laser pulse techniques have opened up a wide variety of applications in both fundamental physics and industrial fields. In this work, $ab$ $initio$ molecular dynamics simulations based on time-dependent density functional theory revealed a steady deceleration of lattice distortion propagation in an aluminum slab with increasing laser pulse intensity. Analysis of the interatomic force revealed a significant reduction in the harmonic terms and non-monotonic growth of anharmonicity. This behavior was characterized by spatially non-uniform force screening by plasmons,…
The theory on the magnetic field energy absorption by metal nanoparticles of a nonspherical shape irradiated with ultrashort laser pulses of different duration is developed. The effect of both the particle surface and the particle shape on the absorbed energy is studied. For the particles having an oblate or prolate spheroidal shape, the dependence of this energy on the orientation of the magnetic field upon a particle, the degree of its deviation from a spherical shape, a pulse duration, and the carrier frequency of the laser ray are found. A significant increase in the absorption is establis…
With the feature of low-power magnetization manipulation at an ultrashort time scale, all optical switching (AOS) has been propelled to the forefront in investigations. To further speed up the magnetization reversal by manipulating ultrashort optical pulses, in this paper, one single square-wave laser pulse (SWLP) vie the combination of heating and Inverse Faraday Effect (IFE) is explored to excite the reversal of magnetization in a Co/Pt system. Simulation results show that the switching time of magnetization is 3 times faster than the using of a traditional Gaussian wave laser pulse (GWLP) u…
The average effective mass of charge carriers produced by an intense ultrashort laser pulse in a transparent solid increases significantly as the excitation mechanism changes from multiphoton transitions to interband tunneling. We theoretically investigate this phenomenon for several dielectrics and semiconductors. For diamond as a representative dielectric, we present a detailed analysis of the laser-induced change of optical properties. When the concentration of free carriers is high, we find that the average effective mass controls not only the intraband charge-carrier transport but also th…
The response of conduction band electrons to a local, pulse-like external excitation is investigated. The charge density wave packets that emerge as a consequence of the excitation leave the interaction region with a speed close to the initial state's band velocity, but there are also oscillations with essentially the same frequency as that of the laser field. As a good estimation, the excitation can also be considered as a localized, time-dependent ponderomotive potential, leading to slowly varying current oscillations. The role of all these effects are investigated for different electron ene…
Reradiation of a spatially non-uniform ultrashort electromagnetic pulse interacting with the linear chain of multielectron atoms is studied in the framework of sudden perturbation approximation. Angular distributions of the reradiation spectrum for arbitrary number of atoms are obtained. It is shown that interference effects for the photon radiation amplitudes lead to appearing of "diffraction" maximums. The obtained results can be extended to the case of two- and three-dimensional crystal lattices and atomic chains. The approach developed allows also to take into account thermal vibrations of…
