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arXiv 0811.2313cond-mat.str-elcond-mat.supr-con
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有机金属与高温$_c$铜酸盐的比较研究

Comparative study of organic metals and high-T$_c$ cuprates

S. Bariši\' c, O. S. Bariši\' c

摘要:

Bechgaard盐和高T $_c$铜酸盐分别用两带和三带模型描述,最低带(几乎)填满一半。在有机物中的相互作用是小的,而在铜酸盐的排斥$U_d$上的Cu网站是最大的能量。在这两种情况下,Mott AF状态在未掺杂的材料中是稳定的。在铜酸盐的金属相中,$U_d\to\infty$极限产生适度的有效排斥。因此,有机物和铜酸盐的金属相中的相干SDW和电荷转移关联的理论是相似的。在(未掺杂的)有机物中,这些相关性与相称的$2k_F$ SDW和$4k_F$键或位点模式有关。相应的模式在金属铜酸盐是无公度SDW,特别是O $_x$/O $_y$四极电荷转移波矢量$2q_{SDW}=q_0+G$。掺杂$x>0$,使费米能级接近范霍夫奇点,他们增强。与晶格的强耦合使静态无公度的O $_x$/O $_y$电荷转移与共线的"X"条纹相关联。与有机物相比,铜酸盐中的相干关联与局部$d_{10}\leftrightarrow d_9$量子电荷转移无序竞争。

英文摘要:

The Bechgaard salts and the high T$_c$ cuprates are described by two and three band models, respectively, with the lowest band (nearly) half filled. In organics the interactions are small, while in cuprates the repulsion $U_d$ on the Cu site is the largest energy. The Mott AF state is stable in undoped materials in both cases. In the metallic phase of cuprates the $U_d\to\infty$ limit produces a moderate effective repulsion. The theories of the coherent SDW and charge-transfer correlations in the metallic phases of organics and cuprates are thus similar. In (undoped) organics those correlations are associated with commensurate $2k_F$ SDW and $4k_F$ bond or site modes. The corresponding modes in metallic cuprates are the incommensurate SDW and in particular O$_x$/O$_y$ quadrupolar charge transfer with wave vector $2q_{SDW}=q_0+G$. They are enhanced for dopings $x>0$, which bring the Fermi level close to the van Hove singularity. Strong coupling to the lattice associates the static incommensurate O$_x$/O$_y$ charge transfer with collinear "nematic" stripes. In contrast to organics, the coherent correlations in cuprates compete with local $d_{10}\leftrightarrow d_9$ quantum charge-transfer disorder.

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