Dark resonances for ground state transfer of molecular quantum gases
Manfred J. Mark, Johann G. Danzl, Elmar Haller, Mattias Gustavsson, Nadia Bouloufa, Olivier Dulieu, Houssam Salami, Tom Bergeman, Helmut Ritsch, Russell Hart, H… 展开作者
Manfred J. Mark, Johann G. Danzl, Elmar Haller, Mattias Gustavsson, Nadia Bouloufa, Olivier Dulieu, Houssam Salami, Tom Bergeman, Helmut Ritsch, Russell Hart, Hanns-Christoph Nägerl
One possible way to produce ultracold, high-phase-space-density quantum gases of molecules in the rovibronic ground state is given by molecule association from quantum-degenerate atomic gases on a Feshbach resonance and subsequent coherent optical multi-photon transfer into the rovibronic ground state. In ultracold samples of Cs_2 molecules, we observe two-photon dark resonances that connect the intermediate rovibrational level |v=73,J=2> with the rovibrational ground state |v=0,J=0> of the singlet $X^1Σ_g^+$ ground state potential. For precise dark resonance spectroscopy we exploit the fact that it is possible to efficiently populate the level |v=73,J=2> by two-photon transfer from the dissociation threshold with the stimulated Raman adiabatic passage (STIRAP) technique. We find that at least one of the two-photon resonances is sufficiently strong to allow future implementation of coherent STIRAP transfer of a molecular quantum gas to the rovibrational ground state |v=0,J=0>.
We propose an experimentally viable setup for the realization of one-dimensional ultracold atom gases in a nanoscale magnetic waveguide formed by two doubly-clamped suspended carbon nanotubes. All common decoherence and atom loss mechanisms are shown to be small. We discuss general consequences of a non-parabolic confinement potential, in particular novel two-body shape resonances, which could be observed in this trap.
Multiparticle entangled states, essential ingredients for modern quantum technologies, are routinely generated in experiments of atomic Bose-Einstein condensates (BECs). However, the entanglement in ultracold interacting Fermi gases has not been yet exploited. In this work, by using an ansatz of composite bosons, we show that many-particle entanglement between two fermionic ensembles localized in spatially separated modes can be generated by splitting an ultracold interacting Fermi gas in the (molecular) BEC regime. This entanglement relies on the fundamental fermion exchange symmetry of molec…
A previously developed approach for the numerical treatment of two particles that are confined in a finite optical-lattice potential and interact via an arbitrary isotropic interaction potential has been extended to incorporate an additional anisotropic dipole-dipole interaction. The interplay of a model but realistic short-range Born-Oppenheimer potential and the dipole-dipole interaction for two confined particles is investigated. A variation of the strength of the dipole-dipole interaction leads to diverse resonance phenomena. In a harmonic confinement potential some resonances show similar…
The molecular association process in a thermal gas of $^{85}$Rb is investigated where the effects of the envelope of the radio-frequency field are taken into account. For experimentally relevant parameters our analysis shows that with increasing pulse length the corresponding molecular conversion efficiency exhibits low-frequency interference fringes which are robust under thermal averaging over a wide range of temperatures. This dynamical interference phenomenon is attributed to Stückelberg phase accumulation between the low-energy continuum states and the dressed molecular state which exhibi…
We discuss the multispecies time-dependent restricted-active-space self-consistent-field theory, an \textit{ab initio} wavefunction-based theory for mixtures of ultracold atomic and molecular gases. We present the general theory, based on the time-dependent variational principle, and derive the equations of motion. The theory captures in a time-dependent setting, via the specification of the restricted-active-space scheme, different levels of approximation from the mean-field to the full configuration interaction approach. To assess its accuracy and to illustrate its ability to identify correl…
We show that the resonance shifts in the fluorescence of a cold gas of rubidium atoms substantially differ from those of thermal atomic ensembles that obey the standard continuous medium electrodynamics. The analysis is based on large-scale microscopic numerical simulations and experimental measurements of the resonance shifts in a steady-state response in light propagation.
We report the observation of resonance-like loss in the trap population of ultracold dysprosium as a function of magnetic field, which we attribute to anisotropy-induced Fano-Feshbach resonances arising from Dy's large magnetic dipole moment and nonzero electronic orbital angular momentum. We recorded these resonances for four different isotopes, three bosonic and one fermionic, over a field range of 0-6 G and show that the number of resonances changes significantly as a function of temperature, even in the nK regime. Most of the observed resonances are of very narrow width. The fermionic isot…
Magnetically tunable Feshbach resonances in ultracold atomic systems are chiefly identified and characterized through time consuming atom loss spectroscopy. We describe an off-resonant dispersive optical probing technique to rapidly locate Feshbach resonances and demonstrate the method by locating four resonances of $^{87}$Rb, between the $|\rm{F} = 1, \rm{m_F}=1 \rangle$ and $|\rm{F} = 2, \rm{m_F}=0 \rangle$ states. Despite the loss features being $\lesssim0.1$ G wide, we require only 21 experimental runs to explore a magnetic field range >18 G, where $1~\rm{G}=10^{-4}$ T. The resonances cons…
We show that an ansatz based on independent composite bosons [Phys. Rep. 463, 215 (2008)] accurately describes the condensate fraction of molecular Bose-Einstein condensates in ultracold Fermi gases. The entanglement between the fermionic constituents of a single Feshbach molecule then governs the many-particle statistics of the condensate, from the limit of strong interaction to close to unitarity. This result strengthens the role of entanglement as the indispensable driver of composite-boson behavior. The condensate fraction of fermion pairs at zero temperature that we compute matches excell…
We introduce, analyze, and compare two novel methods of Single Photon Cooling that generically cool and compress molecular gases. The first method compresses the molecular gas density by three orders of magnitude and increases collision frequency in trapped samples. The second method compresses the phase space density of the gas by at least two orders of magnitude. Designed with combinations of electric and magnetic fields these methods cool the molecules from ~100mK to 1mK using a single irreversible state change. They can be regarded as generic cooling schemes applicable to any molecule with…
We present an analytic model of the refractive index for matter waves propagating through atomic or molecular gases. The model, which combines a WKB treatment of the long range attraction with the Fraunhofer model treatment of the short range repulsion, furnishes a refractive index in compelling agreement with recent experiments of Jacquey et al. [Phys. Rev. Lett. 98, 240405 (2007)] on Li atom matter waves passing through dilute noble gases. We show that the diffractive contribution, which arises from scattering by a two dimensional "hard core" of the potential, is essential for obtaining a co…
A new type of double-resonance spectroscopy of a quantum gas based on interaction-induced frequency modulation of a probe transition has been considered. Interstate interaction of multilevel atoms causes a coherence-dependent collisional shift of the transition between the atomic states |1> and |2> due to a nonzero population of the state |3>. Thus, the frequency of the probe transition |1>-|2> experiences oscillations associated with the Rabi oscillations between the states |1> and |3> under continuous excitation of the drive resonance |1>-|3>. Such a dynamic frequency shift leads to a change…
While many-particle entanglement can be found in natural solids and strongly interacting atomic and molecular gases, generating highly entangled states between weakly interacting particles in a controlled and scalable way presents a significant challenge. We describe here a one-step method to generate entanglement in a dilute gas of cold polar molecules. For molecules in optical traps separated by a few micrometers, we show that maximally entangled states can be created using the strong off-resonant pulses that are routinely used in molecular alignment experiments. We show that the resulting a…
We investigate magnetically tunable Feshbach resonances between ultracold europium atoms and between europium and alkali-metal atoms using multichannel quantum scattering calculations. For ultracold gases of europium atoms both homonuclear $^{153}$Eu+$^{153}$Eu and heteronuclear $^{151}$Eu+$^{153}$Eu systems are studied. Calculations for mixtures of europium and alkali-metal atoms are carried out for prototype systems of $^{153}$Eu+$^{87}$Rb and $^{153}$Eu+$^7$Li. We analyze the prospects for the control of scattering properties, observation of quantum chaotic behavior, and magnetoassociation …
We predict a dynamical resonant effect, which is driven by externally applied linear and quadratic Zeeman fields, in a spin-orbit-coupled spin-1 Bose-Einstein condensate. The Bose-Einstein condensate is assumed to be initialized in some superposed state of Zeeman sublevels and subject to a sudden shift of the trapping potential. It is shown that the time-averaged center-of-mass oscillation and the spin polarizations of the Bose-Einstein condensate exhibit remarkable resonant peaks when the Zeeman fields are tuned to certain strengths. The underlying physics behind this resonance can be traced …
We investigate the prospects of controlling charge-exchange in ultracold collisions of heteroisotopic combinations of atoms and ions of the same element. The treatment, readily applicable to alkali or alkanine-earth metals, is illustrated in the process $^9$Be$^{+}$ + $^{10}$Be $\leftrightarrow$ $^{9}$Be + $^{10}$Be$^{+}$, which exhibits favorable electronic, nuclear, and hyperfine structure. Feshbach resonances are obtained from quantum scattering calculations in a standard coupled-channel formalism with non-BO terms originating from the nuclear kinetic operator. Near a narrow resonance predi…
The dynamics of internal spin, electronic orbital, and nuclear motion states of atoms and molecules have preoccupied the atomic and molecular physics community for decades. Increasingly, such dynamics are being examined within many-body systems composed of atomic and molecular gases. Our findings sometimes bear close relation to phenomena observed in condensed-matter systems, while on other occasions they represent truly new areas of investigation. I discuss several examples of spin dynamics that occur within spinor Bose-Einstein gases, highlighting the advantages of spin-sensitive imaging for…
A superfluid-insulator transition is known to occur in strongly disordered Fermi gases, in both the BCS and BEC regimes; here, we address the properties of this transition across the BEC-BCS crossover. We argue that the critical disorder strength at which superfluidity is lost changes non-monotonically with detuning from Feshbach resonance, and that a reentrant superfluid phase arises for detunings near the fermionic mobility edge. Our analysis of the intermediate regime is quantitatively valid for narrow resonances and near four dimensions, and provides a simple physical picture of this regim…
Many unconventional quantum matters, such as fractional quantum Hall effect and $d$-wave high-Tc superconductor, are discovered in strongly interacting systems. Understanding quantum many-body systems with strong interaction and the unconventional phases therein is one of the most challenging problems in physics nowadays. Cold atom systems possess a natural way to create strong interaction by bringing the system to the vicinity of a scattering resonance. Although this has been a focused topic in cold atom physics for more than a decade, these studies have so far mostly been limited for $s$-wav…
We study the effect of resonances associated with complex molecular interaction of Rydberg atoms on Rydberg blockade. We show that densely-spaced molecular potentials between doubly-excited atomic pairs become unavoidably resonant with the optical excitation at short interatomic separations. Such molecular resonances limit the coherent control of individual excitations in Rydberg blockade. As an illustration, we compute the molecular interaction potentials of Rb atoms near the $100s$ states asymptote to characterize such detrimental molecular resonances, determine the resonant loss rate to mol…
We consider nonlinear spectroscopic effects - interaction-enhanced double resonance and spectrum instability - that appear in ultracold quantum gases owing to collisional frequency shift of atomic transitions and, consequently, due to the dependence of the frequencies on the population of various internal states of the particles. Special emphasis is put to two simplest cases, (a) the gas of two-level atoms and (b) double resonance in a gas of three-level bosons, in which the probe transition frequency remains constant.
