We show that the shear rate at a fixed shear stress in a micellar gel in a jammed state exhibits large fluctuations, showing positive and negative values, with the mean shear rate being positive. The resulting probability distribution functions (PDF's) of the global power flux to the system vary from Gaussian to non-Gaussian, depending on the driving stress and in all cases show similar symmetry properties as predicted by Gallavotti-Cohen steady state fluctuation relation. The fluctuation relation allows us to determine an effective temperature related to the structural constraints of the jammed state. We have measured the stress dependence of the effective temperature. Further, experiments reveal that the effective temperature and the standard deviation of the shear rate fluctuations increase with the decrease of the system size.
We present a simple model to account for the rheological behavior observed in recent experiments on micellar gels. The model combines attachment-detachment kinetics with stretching due to shear, and shows well-defined jammed and flowing states. The large deviation function (LDF) for the coarse-grained velocity becomes increasingly non-quadratic as the applied force $F$ is increased, in a range near the yield threshold. The power fluctuations are found to obey a steady-state fluctuation relation (FR) at small $F$. However, the FR is violated when $F$ is near the transition from the flowing to t…
Athermal disordered systems can exhibit a remarkable response to an applied oscillatory shear: after a relatively few shearing cycles, the system falls into a configuration that had already been visited in a previous cycle. After this point the system repeats its dynamics periodically despite undergoing many particle rearrangements during each cycle. We study the behavior of orbits as we approach the jamming point in simulations of jammed particles subject to oscillatory shear at fixed pressure and zero temperature. As the pressure is lowered, we find that it becomes more common for the system…
We study dense and highly polydisperse emulsions at droplet volume fractions ϕ>= 0.65. We apply oscillatory shear and observe droplet motion using confocal microscopy. The presence of droplets with sizes several times the mean size dramatically changes the motion of smaller droplets. Both affine and nonaffine droplet motions are observed, with the more nonaffine motion exhibited by the smaller droplets which are pushed around by the larger droplets. Droplet motions are correlated over length scales from one to four times the mean droplet diameter, with larger length scales corresponding to hig…
We numerically study the distributions of global pressure that are found in ensembles of statically jammed and quasistatically sheared systems of bidisperse, frictionless, disks at fixed packing fraction $ϕ$ in two dimensions. We use these distributions to address the question of how pressure increases as $ϕ$ increases above the jamming point $ϕ_J$, $p\sim |ϕ- ϕ_J|^y$. For statically jammed ensembles, our results are consistent with the exponent $y$ being simply related to the power law of the interparticle soft-core interaction. For sheared systems, however, the value of $y$ is consistent wit…
在受到缓慢、稳定剪切的气泡筏中的平均速度分布的测量表明流动状态和堵塞状态之间的共存，类似于对于三维泡沫和乳液所观察到的情况[Elissot { \it et al，}，Phys. Rev. Lett. { \bf 88}，218301（2002）]。对于足够慢的剪切，流动是由非线性拓扑重排产生的。我们的报告之间的连接，这种短期运动的泡沫和长期的平均值。我们发现，个别重排事件的速度分布波动，但一个平稳的，平均速度后，达到平均只有相对较少的事件。
It is well known that jammed soft materials will flow if sheared above their yield stress - think mayonnaise spread on bread - but a complete microscopic description of this seemingly sim- ple process has yet to emerge. What remains elusive is a microscopic framework that explains the macroscopic flow, derived from a 3-D spatially resolved analysis of the dynamics of the droplets or particles that compose the soft material. By combining confocal-rheology experiments on compressed emulsions and numerical simulations, we unravel that the primary microscopic mechanisms for flow are strongly influ…
By minimizing the enthalpy of packings of frictionless particles, we obtain jammed solids at desired pressures and hence investigate the jamming transition with and without shear. Typical scaling relations of the jamming transition are recovered in both cases. In contrast to systems without shear, shear-driven jamming transition occurs at a higher packing fraction and the jammed solids are more rigid with an anisotropic force network. Furthermore, by introducing the macro-friction coefficient, we propose an explanation of the packing fraction gap between sheared and non-sheared systems at fixe…
The interplay between shear band (SB) formation and boundary conditions (BC) is investigated in wormlike micellar systems (CPyCl--NaSal) using ultrasonic velocimetry coupled to standard rheology in Couette geometry. Time-resolved velocity profiles are recorded during transient strain-controlled experiments in smooth and sand-blasted geometries. For stick BC standard SB is observed, although depending on the degree of micellar entanglement temporal fluctuations are reported in the highly sheared band. For slip BC wall slip occurs only for shear rates larger than the start of the stress plateau.…
Wall slip, shear banding, and instability in the flow of a triblock copolymer micellar solution
本文研究了三嵌段共聚物胶束溶液（PEO-PPO-PEOPuronicP 84盐水溶液）在同心圆柱体中的剪切流动。我们专注于两个不同的温度低于和高于转变温度$T_c$，这是以前与应力平台的流动曲线中的幻影。(i)在$T=37.0^\circ$ C $<T_c$，整体流量保持均匀和牛顿样，尽管在转子处测量到显著的壁滑移，其可以与流量曲线中的一个反作用点相关联。(ii)在$T=39.4^\circ$ C $>T_c$下，应力平台对应于固定剪切带状态，其特征在于靠近壁的两个高剪切速率带和非常弱的剪切中心带，以及转子处的大滑移速度。在这两种情况下，流动曲线的高剪切分支的特征在于流动不稳定性。根据最近的理论模型和实验，提出了壁滑移、三能带结构和不稳定性的解释。
Memory encoding by cyclic shear is a reliable process to store information in jammed solids, yet its underlying mechanism and its connection to the amorphous structure are not fully understood. When a jammed sphere packing is repeatedly sheared with cycles of the same strain amplitude, it optimizes its mechanical response to the cyclic driving and stores a memory of it. We study memory by cyclic shear training as a function of the underlying stability of the amorphous structure in marginally stable and highly stable packings, the latter produced by minimizing the potential energy using both po…
We analyze fluctuations of particle displacements and stresses in a sheared athermal suspension of elastic capsules (red blood cells). Upon variation of the volume fraction from the dilute up to the highly concentrated regime, our numerical simulations reveal different characteristic power-law regimes of the fluctuation variances and relaxation times. In the jammed phase and at high shear rates, anomalous scaling exponents are found that deviate from pure dimensional predictions. The observed behavior is rationalized via kinetic arguments and a dissipation balance model that takes into account…
Amorphous packings of spheres have been intensely investigated in order to understand the mechanical and flow behaviour of dense granular matter, and to explore universal aspects of the transition from fluid to structurally arrested or jammed states. Considerable attention has recently been focussed on anisotropic packings of frictional grains generated by shear deformation leading to shear jamming, which occurs below the jamming density for isotropic packings of frictionless grains. With the aim of disentangling the role of shear deformation induced structures and friction in generating shear…
In this work, we use flow visualization and rheometry techniques to study the dynamics and evolution of secondary flows in a model wormlike micellar solution sheared between concentric cylinders, i.e., in a Taylor-Couette (TC) cell. The wormlike micellar solution studied in this work contains cetyltrimethylammonium bromide (CTAB) and sodium salicylate (NaSal). This system can be shear banding and highly elastic, non-shear banding and moderately elastic, or nearly Newtonian as the temperature is varied over a narrow range. The effect of elasticity on transitions and instabilities is probed by c…
The impacts of granular jets for both frictional and frictionless grains in two dimensions are numerically investigated. A dense flow with a dead zone emerges during the impact. From our two-dimensional simulation, we evaluate the equations of state and the con- stitutive equations of the flow. The asymptotic divergences of pressure and shear stress similar to the situation near the jamming transition appear for the frictionless case, while their exponents are smaller than those of the sheared granular systems, and are close to the extrapolation from the kinetic theoretical regime. In a simila…
Dry granular materials such as sand, gravel, pills, or agricultural grains, can become rigid when compressed or sheared. At low density, one can distort the shape of a container of granular material without encountering any resistance. Under isotropic compression, the material will reach a certain {\it jamming} density and then resist further compression. {\em Shear jamming} occurs when resistance to shear emerges in a system at a density lower than the jamming density, and the elastic properties of such states have important implications for industrial and geophysical processes. We report on …
We describe experiments that probe the evolution of shear jammed states, occurring for packing fractions $ϕ_S \leq ϕ\leq ϕ_J$, for frictional granular disks, where above $ϕ_J$ there are no stress-free static states. We use a novel shear apparatus that avoids the formation of inhomogeneities known as shear bands. This fixed $ϕ$ system exhibits coupling between the shear strain, $γ$, and the pressure, $P$, which we characterize by the `Reynolds pressure', and a `Reynolds coefficient', $R(ϕ) = (\partial ^2 P/\partial γ^2)/2$. $R$ depends only on $ϕ$, and diverges as $R \sim (ϕ_c - ϕ)^α$, where $ϕ…
Using an athermal quasistatic simulation protocol, we study the distribution of free volumes in sheared hard-particle packings close to, but below, the random-close packing threshold. We show that under shear, and independent of volume fraction, the free volumes develop features similar to close-packed systems -- particles self-organize in a manner as to mimick the isotropically jammed state. We compare athermally sheared packings with thermalized packings and show that thermalization leads to an erasure of these structural features. The temporal evolution, in particular the opening-up and the…
We study the jamming phase diagram of sheared granular material using a novel Couette shear set-up with multi-ring bottom. The set-up uses small basal friction forces to apply a volume-conserving linear shear with no shear band to a granular system composed of frictional photoelastic discs. The set-up can generate arbitrarily large shear strain due to its circular geometry, and the shear direction can be reversed, allowing us to measure a feature that distinguishes shear-jammed from fragile states. We report systematic measurements of the stress, strain and contact network structure at phase b…
Much recent effort has focused on glassy and jamming properties of spherical particles. Very little is known about such phenomena for non-spherical particles, and we take a first step by studying ellipses. We find important differences between the dynamical and structural properties of disks and two-dimensional ellipses subject to continuous Couette shear. In particular, ellipses show slow dynamical evolution, without a counterpart in disks, in the mean velocity, local density, orientational order, and local stress. starting from an unjammed state, ellipses can first jam under shear, and then …
We describe a technique coupling standard rheology and ultrasonic imaging with promising applications to characterization of soft materials under shear. Plane wave imaging using an ultrafast scanner allows to follow the local dynamics of fluids sheared between two concentric cylinders with frame rates as high as 10,000 images per second, while simultaneously monitoring the shear rate, shear stress, and viscosity as a function of time. The capacities of this "rheo-ultrasound" instrument are illustrated on two examples: (i) the classical case of the Taylor-Couette instability in a simple viscous…
Self-organization, and transitions from reversible to irreversible behaviour, of interacting particle assemblies driven by externally imposed stresses or deformation is of interest in comprehending diverse phenomena in soft matter. They have been investigated in a wide range of systems, such as colloidal suspensions, glasses, and granular matter. In different density and driving regimes, such behaviour is related to yielding of amorphous solids, jamming, and memory formation, \emph{etc.} How these phenomena are related to each other has not, however, been much studied. In order to obtain a uni…
We investigate the transient dynamics of a sheared suspension of neutrally buoyant particles under pressure-imposed conditions, subject to a sudden change in shear rate or external pressure. Discrete Element Method simulations show that, depending on the flow parameters (particle and system size, initial volume fraction), the early stress response of the suspension may strongly differ from the prediction of the Suspension Balance Model based on the steady-state rheology. We show that a two-phase model incorporating the Reynolds-like dilatancy law of Pailha & Pouliquen (2009), which prescribes …
