An increase in the dimension of state space for quantum key distribution (QKD) can decrease its fidelity requirements while also increasing its bandwidth. A significant obstacle for QKD with qudits (d>2) has been an efficient and practical quantum state sorter for photons whose complex fields are modulated in both amplitude and phase. We propose such a sorter based on a multiplexed thick hologram, constructed e.g. from photo-thermal refractive (PTR) glass. We validate this approach using coupled-mode theory with parameters consistent with PTR glass to simulate a holographic sorter. The model assumes a three-dimensional state space spanned by three tilted planewaves. The utility of such a sorter for broader quantum information processing applications can be substantial.
We discuss a new method for realizing number-resolving and non-demolition photo detectors by strong coupling of light to individual single photon emitters, which act as strong optical non-linearities. As a specific application we show how these elements can be integrated into an error-proof Bell state analyzer, whose efficiency exceeds the best possible performance with linear optics even for a modest atom-field coupling. The methods are error-proof in the sense that every detection event unambiguously projects the photon state onto a Fock or Bell state.
Photons occupying multiple spatial modes hold a great promise for implementing high-dimensional quantum communication. We use spontaneous four-wave mixing to generate multimode photon pairs in a few mode fiber. We show the photons are correlated in the fiber mode basis using an all-fiber mode sorter. Our demonstration offers an essential building block for realizing high-dimensional quantum protocols based on standard, commercially available fibers, in an all-fiber configuration.
We experimentally demonstrate a programmable parametric mode sorter of high-dimensional signals in a composite spatiotemporal Hilbert space through mode-selective quantum frequency up-conversion. As a concrete example and with quantum communication applications in mind, we consider the Laguerre-Gaussian and Hermite-Gaussian modes as the spatial and temporal state basis for the signals, respectively. By modulating the spatiotemporal profiles of the up-conversion pump, we demonstrate the faithful selection of single photons in those modes and their superposition modes. Our results show an improv…
Photons do not interact directly with each other, but conditional control of one beam by another can be achieved with non-linear optical media at high field intensities. It is exceedingly difficult to reach such intensities at the single photon level but proposals have been made to obtain effective interactions by scattering photons from single transitions. We report here effective interactions between photons created using a quantum dot weakly coupled to a cavity. We show that a passive single-photon non-linearity can modify the counting statistics of a Poissonian beam, sorting the photons in…
Single photons with orbital angular momentum (OAM) have attracted substantial attention from researchers. A single photon can carry infinite OAM values theoretically. Thus, OAM photon states have been widely used in quantum information and fundamental quantum mechanics. Although there have been many methods for sorting quantum states with different OAM values, the nondestructive and efficient sorter of high-dimensional OAM remains a fundamental challenge. Here, we propose a scalable OAM sorter which can categorize different OAM states simultaneously, meanwhile, preserving both OAM and spin ang…
We present an in principle lossless sorter for radial modes of light, using accumulated Gouy phases. The experimental setups have been found by a computer algorithm, and can be intuitively understood in a geometric way. Together with the ability to sort angular-momentum modes, we now have access to the complete 2-dimensional transverse plane of light. The device can readily be used in multiplexing classical information. On a quantum level, it is an analog of the Stern-Gerlach experiment -- significant for the discussion of fundamental concepts in quantum physics. As such, it can be applied in …
The dimension of the state space for information encoding offered by the transverse structure of light is usually limited by the finite size of apertures. The widely used orbital angular momentum (OAM) number of Laguerre-Gaussian (LG) modes in free-space communications cannot achieve the theoretical maximum transmission capacity unless the radial degree of freedom is multiplexed into the protocol. While the methodology to sort the radial quantum number has been developed, the application of radial modes in quantum communications requires an additional ability to efficiently measure the superpo…
High-dimensional encoding schemes have emerged as a novel way to perform quantum information tasks. For high dimensionality, temporal and transverse spatial modes of photons are the two paradigmatic degrees of freedom commonly used in such experiments. Nevertheless, general devices for multi-outcome measurements are still needed to take full advantage of the high-dimensional nature of encoding schemes. We propose a general full-field mode sorting scheme consisting only of up to two optimized phase elements based on evolutionary algorithms that allows for joint sorting of azimuthal and radial m…
The Laguerre-Gaussian (LG) modes constitute a complete basis set for representing the transverse structure of a {paraxial} photon field in free space. Earlier workers have shown how to construct a device for sorting a photon according to its azimuthal LG mode index, which describes the orbital angular momentum (OAM) carried by the field. In this paper we propose and demonstrate a mode sorter based on the fractional Fourier transform (FRFT) to efficiently decompose the optical field according to its radial profile. We experimentally characterize the performance of our implementation by separati…
Recent work considered the ultimate (quantum) limit of the precision of estimating the distance between two point objects. It was shown that the performance gap between the quantum limit and that of ideal continuum image-plane direct detection is the largest for highly sub-Rayleigh separation of the objects, and that a pre-detection mode sorting could attain the quantum limit. Here we extend this to a more general problem of estimating the length of an incoherently radiating extended (line) object. We find, as expected by the Rayleigh criterion, the Fisher information (FI) per integrated photo…
Measuring the state of a quantum system is a fundamental process in quantum mechanics and plays an essential role in quantum information and quantum technologies. One method to measure a quantum observable is to sort the system in different spatial modes according to the measured value, followed by single-particle detectors on each mode. Examples of quantum sorters are polarizing beam-splitters (PBS) -- which direct photons according to their polarization -- and Stern-Gerlach devices. Here we propose a general scheme to sort a quantum system according to the value of any $d$-dimensional degree…
Single-photon wave packets can carry quantum information between nodes of a quantum network. An important general operation in photon-based quantum information systems is blind reversal of a photon's temporal wave-packet envelope, that is, the ability to reverse an envelope without knowing the temporal state of the photon. We present an all-optical means for doing so, using nonlinear-optical frequency conversion driven by a short pump pulse. This scheme allows for quantum operations such as a temporal-mode parity sorter. We also verify that the scheme works for arbitrary states (not only singl…
We describe a mode sorter for two-dimensional parity of transverse spatial states of light based on an out-of-plane Sagnac interferometer. Both Hermite-Gauss (HG) and Laguerre-Gauss (LG) modes can be guided into one of two output ports according to the two-dimensional parity of the mode in question. Our interferometer sorts HG_nm input modes depending upon whether they have even or odd order n+m; it equivalently sorts LG modes depending upon whether they have an even or odd value of their orbital angular momentum. It functions efficiently at the single-photon level, and therefore can be used t…
Classically, electromagnetic pulses are described by real fields that couple to charged matter and propagate causally. We will show here that real fields of the form used in standard classical electromagnetic theory have a quantum mechanical interpretation in which the probability density for a photon to be at x is positive definite and operators representing all of the standard physical observables exist. A covariant alternative to the ω_{k}^{1/2} dependence that appears in most (but not all) presentations of quantum optics and quantum field theory is presented and real scalar one photon adva…
We present an experiment where two photonic systems of arbitrary dimensions can be entangled. The method is based on spontaneous parametric down conversion with trains of d pump pulses with a fixed phase relation, generated by a mode-locked laser. This leads to a photon pair created in a coherent superposition of $d$ discrete emission times, given by the successive laser pulses. Entanglement is shown by performing a two-photon interference experiment and by observing the visibility of the interference fringes increasing as a function of the dimension d. Factors limiting the visibility, such as…
We show that, although the amount of mutual entanglement of photons propagating in free space is fixed, the type of correlations between the photons that determine the entanglement can dramatically change during propagation. We show that this amounts to a migration of entanglement in Hilbert space, rather than real space. For the case of spontaneous parametric down conversion, the migration of entanglement in transverse coordinates takes place from modulus to phase of the bi-photon state and back again. We propose an experiment to observe this migration in Hilbert space and to determine the fu…
Photonics has become a mature field of quantum information science, where integrated optical circuits offer a way to scale the complexity of the setup as well as the dimensionality of the quantum state. On photonic chips, paths are the natural way to encode information. To distribute those high-dimensional quantum states over large distances, transverse spatial modes, like orbital angular momentum (OAM) possessing Laguerre Gauss modes, are favourable as flying information carriers. Here we demonstrate a quantum interface between these two vibrant photonic fields. We create three-dimensional pa…
We test experimentally the quantum ``paradox'' proposed by Lucien Hardy in 1993 [Phys. Rev. Lett. 71, 1665 (1993)] by using single photons instead of photon pairs. This is achieved by addressing two compatible degrees of freedom of the same particle, namely its spin angular momentum, determined by the photon polarization, and its orbital angular momentum, a property related to the optical transverse mode. Because our experiment involves a single particle, we cannot use locality to logically enforce non-contextuality, which must therefore be assumed based only on the observables' compatibility.…
We propose a procedure for defining all single-photon observables in terms of Positive-Operator Valued Measures (POVMs), in particular spin and position. We identify the suppression of $0$-helicity photon states as a projection from an extended Hilbert space onto the photon Hilbert space. We show that all single-photon observables are in general described by POVMs, obtained by applying this projection to opportune Projection-Valued Measures (PVMs), defined on the extended Hilbert space. The POVMs associated to momentum and helicity reduce to PVMs, unlike those associated to position and spin, …
High-dimensional degrees of freedom of photons can encode more quantum information than their two-dimensional counterparts. While the increased information capacity has advantages in quantum applications (such as quantum communication), controlling and manipulating these systems has been challenging. Here we show a method to perform lossless arbitrary high-dimensional Pauli-X gates for single photon. The X-gate consists of a cyclic permutation of qudit basis vectors, and, together with the Z gate, forms the basis for performing arbitrary transformations. We propose an implementation of such ga…
A photon with a modulated wavefront can produce a quantum communication channel in a larger Hilbert space. For example, higher dimensional quantum key distribution (HD-QKD) can encode information in the transverse linear momentum (LM) or orbital angular momentum (OAM) modes of a photon. This is markedly different than using the intrinsic polarization of a photon. HD-QKD has advantages for free space QKD since it can increase the communication channelÕs tolerance to bit error rate (BER) while maintaining or increasing the channels bandwidth. We describe an efficient numerical simulation of the …
Many quantum key distribution analyses examine the link security in a subset of the full Hilbert space that is available to describe the system. In reality, information about the photon state can be embedded in correlations between the polarization space and other dimensions of the Hilbert space in such a way that Eve can determine the polarization of a photon without affecting it. This paper uses the concept of suitability to quantify the available information for Eve, and then describe a systematic way to calculate and measure these possibilities.
Photonic-Implemented Efficient Deep Quantum Neural Network via Virtual-Driven Hilbert Space Expansion
College of Information Science and Electronic Engineering and ZJU-Hangzhou Global Scientific and Technological Innovation Center, Zhejiang University（浙江大学信息与电子工程学院及浙大杭州全球科创中心）
Quantum key distributions (QKD) systems often rely on polarization of light for encoding, thus limiting the amount of information that can be sent per photon and placing tight bounds on the error that such a system can tolerate. Here we describe a proof-of-principle experiment that indicates the feasibility of high-dimensional QKD based on the transverse structure of the light field, allowing for the transfer of more than 1 bit per photon. Our implementation uses the orbital angular momentum (OAM) of photons and the corresponding mutually unbiased basis of angular position (ANG). Our experimen…
Building an efficient quantum memory in high-dimensional Hilbert spaces is one of the fundamental requirements for establishing high-dimensional quantum repeaters, where it offers many advantages over two-dimensional quantum systems, such as a larger information capacity and enhanced noise resilience. To date, there have been no reports about how to achieve an efficient high-dimensional quantum memory. Here, we experimentally realize a quantum memory that is operational in Hilbert spaces of up to 25 dimensions with a storage efficiency of close to 60%. The proposed approach exploits the spatia…
The practically useful criteria of separable states $ρ=\sum_{k}w_{k}ρ_{k}$ in $d=2\times2$ are discussed. The equality $G({\bf a},{\bf b})= 4[\langle ψ|P({\bf a})\otimes P({\bf b})|ψ\rangle-\langle ψ|P({\bf a})\otimes{\bf 1}|ψ\rangle\langle ψ|{\bf 1}\otimes P({\bf b})|ψ\rangle]=0$ for any two projection operators $P({\bf a})$ and $P({\bf b})$ provides a necessary and sufficient separability criterion in the case of a separable pure state $ρ=|ψ\rangle\langleψ|$. We propose the separability criteria of mixed states, which are given by ${\rm Tr}ρ\{{\bf a}\cdot {\bf σ}\otimes {\bf b}\cdot {\bf σ}\…
Exploiting hyperentanglement of photon pairs, that is, simultaneous entanglement in multiple degrees of freedom(DOFs), increases the dimensionality of Hilbert spaces for quantum information processing. However, generation of hyperentangled photon pairs collinearlly, while produces high brightness, results in a smaller Hilbert space due to the two photons being in the same spatial mode. In this letter, we point out that one can recover the full dimensionality of such hyperentanglement through a simple interference set up, similar to the time-reversed Hong-Ou-Mandel (TR-HOM) process. Different f…
We propose a novel setup to investigate the quantum non-locality of orbital angular momentum states living in a high-dimensional Hilbert space. We incorporate non-integer spiral phase plates in spatial analyzers, enabling us to use only two detectors. The resulting setup is somewhat reminiscent of that used to measure polarization entanglement. However, the two-photon states that are produced, are not confined to a 2X2-dimensional Hilbert space, and the setup allows the probing of correlations in a high-dimensional space. For the special case of half-integer spiral phase plates, we predict a v…
We present an experimental implementation of optimum measurements for quantum state discrimination. Optimum maximum-confidence discrimination and optimum unambiguous discrimination of two mixed single-photon polarization states were performed. For the latter the states of rank two in a four-dimensional Hilbert space are prepared using both path and polarization encoding. Linear optics and single photons from a true single-photon source based on a semiconductor quantum dot are utilized.
The mechanism of describing quantum states by standard probability (tomographic one) instead of wave function or density matrix is elucidated. Quantum tomography is formulated in an abstract Hilbert space framework, by means of the identity decompositions in the Hilbert space of hermitian linear operators, with trace formula as scalar product of operators. Decompositions of identity are considered with respect to over-complete families of projectors labeled by extra parameters and containing a measure, depending on these parameters. It plays the role of a Gram-Schmidt orthonormalization kernel…
Spatially entangled twin photons allow the study of high-dimensional entanglement, and the Laguerre-Gauss modes are the most commonly used basis to discretize the single photon mode spaces. In this basis, to date only the azimuthal degree of freedom has been investigated experimentally due to its fundamental and experimental simplicity. We show that the full spatial entanglement is indeed accessible experimentally, i.e., we have found practicable radial detection modes with negligible cross correlations. This allows us to demonstrate hybrid azimuthal -- radial quantum correlations in a Hilbert…
We present a protocol for deterministic and highly efficient quantum cryptography with entangled photon pairs in a 4x4-dimentional Hilbert space. Two communicating parties, Alice and Bob first share a both polarization- and path-entangled photon pair, and then each performs a complete Bell-state measurement on their own photon in one of two complementary Bell-state bases. It is demonstrated that each measurement in which both Alice and Bob register a photon can build certain perfect correlation and generate 1.5 key bits on average. The security of our protocol is guaranteed by the non-cloning …
Coherent states in a projected Hilbert space have many useful properties. When there are conserved quantities, a representation of the entire Hilbert space is not necessary. The same issue arises when conditional observations are made with post-selected measurement results. In these cases, only a part of the Hilbert space needs to be represented, and one can define this restriction by way of a projection operator. Here coherent state bases and normally-ordered phase-space representations are introduced for treating such projected Hilbert spaces, including existence theorems and dynamical equat…
One of the most important properties of orbital angular momentum (OAM) of photons is that the Hilbert space required to describe a general quantum state is infinite dimensional. In principle, this could allow for encoding arbitrarily large amounts of quantum information per photon, but in practice, this potential is limited by decoherence and errors. To determine whether photons with OAM are suitable for quantum communication, we numerically simulated their passage through a turbulent atmosphere and the resulting errors. We also proposed an encoding scheme to protect the photons from these err…
We propose an interferometric method for statistically discriminating between nonorthogonal states in high dimensional Hilbert spaces for use in quantum information processing. The method is illustrated for the case of photon orbital angular momentum (OAM) states. These states belong to pairs of bases that are mutually unbiased on a sequence of two-dimensional subspaces of the full Hilbert space, but the vectors within the same basis are not necessarily orthogonal to each other. Over multiple trials, this method allows distinguishing OAM eigenstates from superpositions of multiple such eigenst…
We experimentally investigate the properties of hyperentangled states displaying simultaneous entanglement in multiple degrees of freedom, and find that Bell tests beyond the standard Clauser, Horne, Shimony, Holt inequality can reveal a higher-dimensional nature in a device-independent way. Specifically, we show that hyperentangled states possess more than just simultaneous entanglement in separate degrees of freedom but also entanglement in a higher dimensional Hilbert space. We also verify the steerability of hyperentangled quantum states by steering different photonic degrees of freedom.
We propose a multidimensional quantum information encoding approach based on temporal modulation of single photons, where the Hilbert space can be spanned by an in-principle infinite set of orthonormal temporal profiles. We analyze two specific realizations of such modulation schemes, and show that error rate per symbol can be smaller than 1% for practical implementations. Temporal modulation may enable multidimensional quantum communication over the existing fiber optical infrastructure, as well as provide an avenue for probing high-dimensional entanglement approaching the continuous limit.
We experimentally demonstrate the first quantum system entangled in every degree of freedom (hyperentangled). Using pairs of photons produced in spontaneous parametric downconversion, we verify entanglement by observing a Bell-type inequality violation in each degree of freedom: polarization, spatial mode and time-energy. We also produce and characterize maximally hyperentangled states and novel states simultaneously exhibiting both quantum and classical correlations. Finally, we report the tomography of a 2x2x3x3 system (36-dimensional Hilbert space), which we believe is the first reported ph…
We present a new implementation of the BB84 quantum key distribution protocol that employs a $d$-dimensional Hilbert space spanned by spatial modes of the propagating beam that have a definite value of orbital angular momentum. Each photon carries $\log d$ bits of information, increasing the key generation rate of the protocol. The states used in the transmission part of the protocol are invariant under rotations about the propagation direction, making this implementation independent of the alignment between the reference frames of the sender and receiver. The protocol still works when these r…
Field-orthogonal temporal modes of photonic quantum states provide a new framework for quantum information science (QIS). They intrinsically span a high-dimensional Hilbert space and lend themselves to integration into existing single-mode fiber communication networks. We show that the three main requirements to construct a valid framework for QIS -- the controlled generation of resource states, the targeted and highly efficient manipulation of temporal modes and their efficient detection -- can be fulfilled with current technology. We suggest implementations of diverse QIS applications based …
Spontaneous collapse models of state vector reduction represent a possible solution to the quantum measurement problem. In the present paper we focus our attention on the Ghirardi-Rimini-Weber (GRW) theory and the corresponding continuous localisation models in the form of a Brownian-driven motion in Hilbert space. We consider experimental setups in which a single photon hits a beam splitter and is subsequently detected by photon detector(s), generating a superposition of photon-detector quantum states. Through a numerical approach we study the dependence of collapse times on the physical feat…
We investigate coherence in one- and two-photon optical systems, both theoretically and experimentally. In the first case, we develop the density operator representing a single photon state subjected to a non-dissipative coupling between observed (polarization) and unobserved (frequency) degrees of freedom. We show that an implementation of ``bang-bang'' quantum control protects photon polarization information from certain types of decoherence. In the second case, we investigate the existence of a "decoherence-free" subspace of the Hilbert space of two-photon polarization states under the acti…
A 6-qubit hyperentangled state has been realized by entangling two photons in three degrees of freedom. These correspond to the polarization, the longitudinal momentum and the indistinguishable emission produced by a 2-crystal system operating with Type I phase matching in the spontaneous parametric down conversion regime. The state has been characterized by a chained interferometric apparatus and its complete entangled nature has been tested by a novel witness criterium specifically introduced for hyperentangled states. The experiment represents the first realization of a genuine hyperentangl…
We present the first robust implementation of a coined quantum walk over five steps using only passive optical elements. By employing a fiber network loop we keep the amount of required resources constant as the walker's position Hilbert space is increased. We observed a non-Gaussian distribution of the walker's final position, thus characterizing a faster spread of the photon wave-packet in comparison to the classical random walk. The walk is realized for many different coin settings and initial states, which opens the way for the implementation of a quantum walk-based search algorithm.
This paper gives a constructive answer to the question whether photon states can contain or not, and to what extent, the readings of rulers and clocks. The paper first shows explicitly that, along with the momentum representation, there is room in the one photon Hilbert space for an alternative position representation. This is made possible by the existence of a self-adjoint, involutive, position operator conjugate to the momentum operator (due to M. Hawton). Position and momenta are shown to satisfy the Heisenberg-Weyl quantization rules in the helicity basis, which is analyzed anew from this…
Within the framework of exact quantum electrodynamics in dispersing and absorbing media, we have studied the quantum state of the radiation emitted from an initially in the upper state prepared two-level atom in a high-$Q$ cavity, including the regime where the emitted photon belongs to a wave packet that simultaneously covers the areas inside and outside the cavity. For both continuing atom--field interaction and short-term atom--field interaction, we have determined the spatio-temporal shape of the excited outgoing wave packet and calculated the efficiency of the wave packet to carry a one-p…
In this paper, we study entanglement distillation of multipartite continuous-variable Gaussian entangled states. Following Opatrný \emph{et al.}'s photon subtraction (PS) scheme, the probability of successful distillation decreases exponentially with the number of parties $N$. However, here, we shall propose an entanglement distillation scheme whose success probability scales as a constant with $N$. Our protocol employs several local squeezers, but it requires only a single PS operation. Using the logarithmic negativity as a measure of entanglement, we find that both the success probability an…
We demonstrate that a single-photon field modulated with n different pseudorandom phase sequences (PPSs) can constitute a 2^n-dimensional Hilbert space that contains tensor product structure. By using the single photon field modulated with PPSs, we discuss effective simulation of Bell states and GHZ state, and apply both correlation analysis and von Neumann entropy to characterize the simulation. We obtain similar results with the cases in quantum mechanics and find that the conclusions can be easily generalized to n quantum particles. The research on simulation of quantum entanglement may be …
We design a scheme for detecting a single photon loss from multi-modal quantum signals transmitted via a fiber or in free space. This consists of a special type of unitary coding transformation, the controlled-squeezing, applied prior to the transmission on the signal composed by information and ancilla modes. At the receiver, the inverse unitary transformation is applied -decoding, and the ancilla modes are measured via photon detection. The outcome reveals whether a photon loss has occurred. Distortion of the information part of the signal caused by an ancilla photon loss can be corrected if…
