Engineering Giant Nonlinearities in Quantum Nanosystems

Giant Kerr nonlinearities in Circuit-QED

The very small size of optical nonlinearities places wide ranging restrictions on the types of novel physics one can explore. For an ensemble of multi-level systems one can synthesize a large effective optical nonlinearity using quantum coherence effects but such non-linearities are technically extremely challenging to demonstrate at the single atom level. In this work we describe how a single artificial multi-level Cooper Pair Box molecule, interacting with a superconducting microwave coplanar waveguide resonator, when suitably driven, can generate extremely large optical nonlinearities at mi…

Cavity-induced giant Kerr nonlinearities in a driven V-type atom

We discuss a simple and experimentally realizable model for creation of enhanced Kerr nonlinearities accompanied by vanishing absorption. The model involves a V-type atom subjected to a strong drive laser, a weak probe laser and coupled to a single-mode cavity field. Working in the bad-cavity limit, we find that the simultaneous coupling of the cavity field to both atomic transitions creates a coherence between the transitions and thus can lead to quantum interference effects. We investigate the influences of the cavity field frequency, the cavity field-atom coupling constants and the atomic d…

Giant optical nonlinearities from Rydberg-excitons in semiconductor microcavities

The realization of exciton-polaritons -- hybrid excitations of semiconductor quantum well excitons and cavity photons -- has been of great technological and scientific significance. In particular, the short-range collisional interaction between excitons has enabled explorations into a wealth of nonequilibrium and hydrodynamical effects that arise in weakly nonlinear polariton condensates. Yet, the ability to enhance optical nonlinearities would enable quantum photonics applications and open up a new realm of photonic many-body physics in a scalable and engineerable solid-state environment. Her…

Giant optical nonlinearity cancellation in quantum wells

Second-order optical nonlinearities can be greatly enhanced by orders of magnitude in resonantly excited nanostructures, theoretically predicted and experimentally investigated in a variety of semiconductor systems. These resonant nonlinearities continually attract attention, particularly in newly discovered materials, but tend not to be as efficient as currently predicted. This limits their exploitation in frequency conversion. Here, we present a clear-cut theoretical and experimental demonstration that the second-order nonlinear susceptibility can vary by orders of magnitude as a result of g…

Realization of a Knill-Laflamme-Milburn C-NOT gate -a photonic quantum circuit combining effective optical nonlinearities

Quantum information science addresses how uniquely quantum mechanical phenomena such as superposition and entanglement can enhance communication, information processing and precision measurement. Photons are appealing for their low noise, light-speed transmission and ease of manipulation using conventional optical components. However, the lack of highly efficient optical Kerr nonlinearities at single photon level was a major obstacle. In a breakthrough, Knill, Laflamme and Milburn (KLM) showed that such an efficient nonlinearity can be achieved using only linear optical elements, auxiliary pho…

光泵浦下强耦合三量子比特波导系统中的缀饰态与量子非线性探测

Probing dressed states and quantum nonlinearities in a strongly coupled three-qubit waveguide system under optical pumping

本文研究光泵浦三量子比特波导的强耦合与非线性光谱，结合介质依赖主方程和 matrix product states 揭示缀饰态、巨原子延迟效应及 Markov 模型局限。