Evidence for Fermi surface reconstruction in the static stripe phase of La$_{1.8-x}$Eu$_{0.2}$Sr$_x$CuO$_{4}$, $x=1/8$
V. B. Zabolotnyy, A. A. Kordyuk, D. S. Inosov, D. V. Evtushinsky, R. Schuster, B. Buechner, N. Wizent, G. Behr, Sunseng Pyon, H. Takagi, R. Follath, S. V. Borisenko
We present a photoemission study of La$_{0.8-x}$Eu$_{0.2}$Sr$_x$CuO$_{4}$ with doping level $x$=1/8, where the charge carriers are expected to order forming static stripes. Though the local probes in direct space seem to be consistent with this idea, there has been little evidence found for such ordering in quasiparticle dispersions. We show that the Fermi surface topology of the 1/8 compound develops notable deviations from that observed for La$_{2- x}$Sr$_x$CuO$_{4}$ in a way consistent with the FS reconstruction expected for the scattering on the antiphase stripe order.
The oxygen isotope effect on the superconductivity, stripe phase and structure transition is systematically investigated in La$_{1.6-x}$Nd$_{0.4}$Sr$_{x}$CuO$_4$ with static stripe phase. Substitution of $^{16}$O by $^{18}$O leads to a decrease in superconducting transition temperature T$_C$, while enhances the temperature of the structural transition from low-temperature-orthorhombic (LTO) phase to low-temperature-tetragonal (LTT) phase. Compared to the Nd free sample, a larger isotope effect on $T_C$ is observed in La$_{1.6-x}$Nd$_{0.4}$Sr$_{x}$CuO$_4$. These results indicate that the distor…
We demonstrate that one can measure the charge-stripe order parameter in the hole-doped CuO(2) planes of La(1.875)Ba(0.125)CuO(4), La(1.48)Nd(0.4)Sr(0.12)CuO(4) and La(1.68)Eu(0.2)Sr(0.12)CuO(4) utilizing the wipeout effects of Cu-63 NQR. Application of the same approach to La(2-x)Sr(x)CuO(4) reveals the presence of similar stripe order for the entire underdoped superconducting regime 1/16 < x < 1/8.
Recent spectroscopic observations of a d-wave-like gap in stripe-ordered La(2-x)Ba(x)CuO(4) with x=1/8 have led us to critically analyze the anisotropic transport and magnetization properties of this material. The data suggest that concomitant with the spin ordering is an electronic decoupling of the CuO(2) planes. We observe a transition (or crossover) to a state of two-dimensional (2D) fluctuating superconductivity, which eventually reaches a 2D superconducting state below a Berezinskii-Kosterlitz-Thouless transition. Thus, it appears that the stripe order in La(2-x)Ba(x)CuO(4) frustrates th…
Superstructure reflections due to the ordering of holes into stripes in La_(1.45)Nd_(0.4)Sr_(0.15)CuO_4 have been studied with high energy x-ray diffraction. These reflections have been observed clearly for the first time in a sample which is superconducting at low temperatures (T_c = 10 K). The stripe peaks vanish above 62(5) K whereas the magnetic signal of the stripe ordering which has been seen with neutrons before is already suppressed at 45 K. Our results confirm that the ordering of spins and holes is driven by the charges as it is found in the case of La_(1.6-x)Nd_(0.4)Sr_(x)CuO_(4) at…
Resistivity and magnetization measurements are used for studying the transverse sliding of AF domain boundaries in lightly doped La_{2-x}Sr_{x}CuO_{4}. We discuss that it is the freezing of the transverse boundary motion that is responsible for the appearance of ``spin-glass'' features at low temperatures.
We investigate the transport properties of La$_{1.8-x}$Eu$_{0.2}$Sr$_x$CuO$_4$ ($x=0.04$, 0.08, 0.125, 0.15, 0.2) with a special focus on the Nernst effect in the normal state. Various anomalous features are present in the data. For $x=0.125$ and 0.15 a kink-like anomaly is present in the vicinity of the onset of charge stripe order in the LTT phase, suggestive of enhanced positive quasiparticle Nernst response in the stripe ordered phase. At higher temperature, all doping levels except $x=0.2$ exhibit a further kink anomaly in the LTO phase which cannot unambiguously be related to stripe orde…
Temperature dependence of the Hall coefficient, R_H_, has been investigated in charge-spin stripe-ordered La-214 high-T_c_ superconductors. Using the simplest stripe-ordered system of La_2-x_Ba_x_CuO_4_, it has been clarified that both the behavior of R_H_ and its sign exhibit significant dependences on the hole concentration. That is, R_H_ is zero in the ground state of the charge-spin stripe order at x=1/8, while it is negative in the less-stabilized state of the charge stripe for x<1/8. These are interpreted as owing to the delicate balance of the contributions of the hole-like Fermi surfac…
We investigate the hole and lattice dynamics in a prototypical high temperature superconducting system La{2-x}Sr{x}CuO{4} using infrared spectroscopy. By exploring the anisotropy in the electronic response of CuO2 planes we show that our results support the notion of stripes. Nevertheless, charge ordering effects are not apparent in the phonon spectra. All crystals show only the expected infrared active modes for orthorhombic phases without evidence for additional peaks that may be indicative of static charge ordering. Strong electron-phonon interaction manifests itself through the Fano linesh…
Static stripe order is detrimental to superconductivity. Yet, it has been proposed that transverse stripe fluctuations may enhance the inter-stripe Josephson coupling and thus promote superconductivity. Direct experimental studies of stripe dynamics, however, remain difficult. From a strong-coupling perspective, transverse stripe fluctuations are realized in the form of dynamic "kinks" -- sideways shifting stripe sections. Here, we show how modest uniaxial pressure tuning reorganizes directional kink alignment. Our starting point is La$_{1.88}$Sr$_{0.12}$CuO$_4$, where transverse kink ordering…
We use resonant inelastic x-ray scattering to investigate charge-stripe correlations in La$_{1.675}$Eu$_{0.2}$Sr$_{0.125}$CuO$_4$. By differentiating elastic from inelastic scattering, it is demonstrated that charge-stripe correlations precede both the structural low-temperature tetragonal phase and the transport-defined pseudogap onset. The scattering peak amplitude from charge stripes decays approximately as $T^{-2}$ towards our detection limit. The in-plane integrated intensity, however, remains roughly temperature independent. Therefore, although the incommensurability shows a remarkably l…
Optical excitation of stripe-ordered La$_{2-x}$Ba$_x$CuO$_4$ has been shown to transiently enhance superconducting tunneling between the CuO$_2$ planes. This effect was revealed by a blue-shift, or by the appearance of a Josephson Plasma Resonance in the terahertz-frequency optical properties. Here, we show that this photo-induced state can be strengthened by the application of high external magnetic fields oriented along the c-axis. For a 7-Tesla field, we observe up to a ten-fold enhancement in the transient interlayer phase correlation length, accompanied by a two-fold increase in the relax…
We report on a thermoelectric investigation of the stripe and superconducting phases of the cuprate La$_{2-x}$Ba$_{x}$CuO$_{4}$ near the $x=1/8$ doping known to host stable stripes. We use the doping and magnetic field dependence of field-symmetric Nernst effect features to delineate the phenomenology of these phases. Our measurements are consistent with prior reports of time-reversal symmetry breaking signatures above the superconducting $T_{\rm c}$, and crucially detect a sharp, robust, field-invariant peak at the stripe charge order temperature, $T_{\rm {\scriptscriptstyle CO}}$. Our observ…
We report combined soft and hard x-ray scattering studies of the electronic and lattice modulations associated with stripe order in La$_{1.875}$Ba$_{0.125}$CuO$_4$ and La$_{1.48}$Nd$_{0.4}$Sr$_{0.12}$CuO$_4$. We find that the amplitude of both the electronic modulation of the hole density and the strain modulation of the lattice is significantly larger in La$_{1.875}$Ba$_{0.125}$CuO$_4$ than in La$_{1.48}$Nd$_{0.4}$Sr$_{0.12}$CuO$_4$ and is also better correlated. The in-plane correlation lengths are isotropic in each case; for La$_{1.875}$Ba$_{0.125}$CuO$_4$, $ξ^{hole}=255\pm 5$ Å whereas for…
Low energy spin excitations were investigated in the static stripe phase of La_{2-x}Sr_xCuO_4 using elastic and inelastic neutron scattering on single crystals. For x = 1/8 in which long-range static stripe order exists, an energy gap of E_g = 4 meV exists in the excitation spectrum in addition to strong quasi-elastic, incommensurate spin fluctuations associated with the static stripes. When x increases, the spectral weight of the spin fluctuations shifts from the quasi-elastic continuum to the excitation spectrum above E_g. The dynamic correlation length as a function of energy and the temper…
We have measured the ab-plane resistivity of La$_{2-x}$Sr$_x$CuO$_4$ single crystals with small Sr content (x=0.052 $÷$ 0.075) between 4.2 and 300 K by using the AC Van der Pauw technique. As recently suggested by Ichikawa et al., the deviation from the linearity of the $ρ_{\mathrm{ab}}(T)$ curve starting at a temperature T$_{\mathrm{ch}}$ can be interpreted as due to a progressive slowing down of the fluctuations of pre-formed charge stripes. An electronic transition of the stripes to a more ordered phase could instead be responsible for some very sharp anomalies present in the $ρ_{\mathrm{ab…
Detailed behavior of the magnetoresistance (MR) is studied in lightly doped antiferromagnetic La_{1.99}Sr_{0.01}CuO_{4}, where, thanks to the weak ferromagnetic moment due to spin canting, the antiferromagnetic (AF) domain structure can be manipulated by the magnetic field. The MR behavior demonstrates that CuO_2 planes indeed contain anti-phase AF domain boundaries in which charges are confined, forming anti-phase stripes. The data suggest that a high magnetic field turns the anti-phase stripes into in-phase stripes, and the latter appear to give better conduction than the former, which chall…
Temperature dependence of the in-plane electrical resistivity, $ρ_{\rm ab}$, in various magnetic fields has been measured in the single-crystal La$_{2-x}$Ba$_x$CuO$_4$ with $x=0.08$, 0.10, 0.11 and La$_{1.6-x}$Nd$_{0.4}$Sr$_x$CuO$_4$ with $x=0.12$. It has been found that the superconducting transition curve shows a so-called fan-shape broadening in magnetic fields for $x=0.08$, while it shifts toward the low-temperature side in parallel with increasing field for $x=0.11$ and 0.12 where the charge-spin stripe order is formed at low temperatures. As for $x=0.10$, the broadening is observed in lo…
Interlayer transport in high-$T_C$ cuprates is mediated by superconducting tunneling across the CuO$_2$ planes. For this reason, the terahertz frequency optical response is dominated by one or more Josephson plasma resonances and becomes highly nonlinear at fields for which the tunneling supercurrents approach their critical value, $I_C$. These large terahertz nonlinearities are in fact a hallmark of superconducting transport. Surprisingly, however, they have been documented in La$_{2-x}$Ba$_x$CuO$_4$ also above $T_C$ for doping values near $x=1/8$, and interpreted as an indication of superflu…
Recently Lucarelli {\it et al.} have reported\cite{lucarelli} temperature-dependence of the in-plane optical reflectivity of La$_{2-x}$Sr$_x$CuO$_4$ over a wide doping range, focusing on the infrared peaks at 30 cm$^{-1}$ (for $x$=0.12), 250 cm$^{-1}$ and 510 cm$^{-1}$. They interpreted the first peak (30 cm$^{-1}$) as a signature of charge stripe ordering, while the latter two (250 cm$^{-1}$ and 510 cm$^{-1}$) are attributed to the polaronic charge excitations. However, careful readers would notice that the reported spectra are largely different from those so far measured on the same system. …
Based on the newly developed real-space spin-parallel pairing and superconducting theory, we explore a simple explanation for the observed checkerboard patterns in hole-doped Ca{2-x}Na{x}CuO{2}Cl{2} cuprate superconductor. At a hole concentration x=1/8=0.125, the analytical results show that there exists a phase competition between non-superconducting 4a*4b (a=b) checkerboard phase and 8a*2c superconducting vortex phase, where a, b and c are the lattice constants of the superconductor. At a lower hole concentration x=1/16=0.0625, it is revealed that the metastable 4\sqrt{2}a*4\sqrt{2}a checker…
We present a Cu nuclear magnetic/quadrupole resonance study of the charge stripe ordered phase of LBCO, with detection of previously unobserved ('wiped-out') signal. We show that spin-spin and spin-lattice relaxation rates are strongly enhanced in the charge ordered phase, explaining the apparent signal decrease in earlier investigations. The enhancement is caused by magnetic, rather than charge fluctuations, conclusively confirming the long-suspected assumption that spin fluctuations are responsible for the wipeout effect. Observation of the full Cu signal enables insight into the spin and ch…
Recent angle-resolved $c$-axis resistivity measurements of the stripe-ordered La$_{2-x}$Ba$_x$CuO$_4$ (LBCO) with $x=1/8$ revealed an unexpected dependence on the direction of the in-plane magnetic field. We argue that these and other available data for the $c$-axis transport point to the existence of superconducting pairs of two different types in the $x=1/8$ LBCO below the stripe ordering temperature. The pairs of one type carry finite momentum and are confined to the Cu-O planes; the pairs of other type (probably the conventional $d$-wave with zero momentum) propagate along narrow conductin…
We present new x-ray and neutron scattering measurements of stripe order in La(1.875)Ba(0.125)CuO(4), along with low-field susceptibility, thermal conductivity, and specific heat data. We compare these with previously reported results for resistivity and thermopower. Temperature-dependent features indicating transitions (or crossovers) are correlated among the various experimental quantities. Taking into account recent spectroscopic studies, we argue that the most likely interpretation of the complete collection of results is that an unusual form of two-dimensional superconducting correlations…
In those cases where charge stripe order has been observed in cuprates, the crystal structure is such that the average rotational symmetry of the CuO2 planes is reduced from four-fold to two-fold. As a result, one could argue that the reduced lattice symmetry is essential to the existence of stripe order. We use pressure to restore the average four-fold symmetry in a single crystal of La(1.875)Ba(0.125)CuO(4), and show by x-ray diffraction that charge stripe order still occurs. Thus, electronically-driven stripe order can spontaneously break the lattice symmetry.
Lattice distortions associated with charge stripe order in 1/8 hole-doped La$_{1.875}$Ba$_{0.125-x}$Sr$_{x}$CuO$_{4}$ are studied using synchrotron X-ray diffraction for $x=0.05$ and $x=0.075$. The propagation wave vector and charge order correlation lengths are determined with a high accuracy, revealing that the oblique charge stripes in orthorhombic $x=0.075$ crystal are more disordered than the aligned stripes in tetragonal $x=0.05$ crystal. The twofold periodicity of lattice modulations along the c-axis is explained by long-range Coulomb interactions between holes on neighboring CuO$_{2}$ …
Precise neutron-scattering experiments on La$_{1.88-y}$Sr$_{0.12+y}$Cu$_{0.99}$R$_{0.01}$O$_4$ ($y$=0 for R=Cu, Zn and $y$=0.01 for R=Ga, Fe) were performed to examine the stability of stripe order in cuprate oxides through impurity substitution effects. For all the impurity-substituted samples a static charge-density-wave order similar to that reported in the low-temperature-tetragonal phase (LTT) was discovered in the low-temperature-orthorhombic (LTO) phase for the first time. Fe substitution significantly enhanced both the charge- and spin-density-wave orders. These results indicate that d…
The dynamical stripe structure relating to the "1/8 problem" was investigated in La$_{2-x}$Sr$_x$CuO$_4$ utilizing the high frequency response of Raman scattering. The split of the two-magnon peak due to the formation of the stripe structure was observed at whole Sr concentration region from $x=0.035$ to 0.25 at low temperatures. Especially clear split was observed at low carrier concentration region $x=0.035 - 0.06$ and at $x \sim 1/8$. The onset temperatures of these stripe structures are as high as 300-350 K, which are much higher than the temperatures measured by slow response probes.
We show that disruption of charge-density-wave (stripe) order by charge transfer excitation, enhances the superconducting phase rigidity in La_{1.885}Ba_{0.115}CuO_4 (LBCO). Time-Resolved Resonant Soft X-Ray Diffraction demonstrates that charge order melting is prompt following near-infrared photoexcitation whereas the crystal structure remains intact for moderate fluences. THz time-domain spectroscopy reveals that, for the first 2 ps following photoexcitation, a new Josephson Plasma Resonance edge, at higher frequency with respect to the equilibrium edge, is induced indicating enhanced superc…
Comment on "Light-induced melting of competing stripe orders without introducing superconductivity in La$_{1.875}$Ba$_{0.125}$CuO$_4$" (arXiv:2306.07869v1)
Recent neutron diffraction studies have yielded evidence that, in a particular cuprate family, holes doped into the CuO(2) planes segregate into stripes that separate antiferromagnetic domains. Here it is shown that such a picture provides a quantitatively consistent interpretation of the spin fluctuations measured by neutron scattering in La(1.85)Sr(0.15)CuO(4) and YBa(2)Cu(3)O(6+x).
We present the results of neutron-scattering studies on various aspects of crystalline and magnetic structure in single crystals of La(1.6-x)Nd(0.4)Sr(x)CuO(4) with x=0.12 and 0.15. In particular, we have reexamined the degree of stripe order in an x=0.12 sample. Measurements of the width for an elastic magnetic peak show that it saturates at a finite value below 30 K, corresponding to a spin-spin correlation length of 200 A. A model calculation indicates that the differing widths of magnetic and (previously reported) charge-order peaks, together with the lack of commensurability, can be consi…
The discovery of charge- and spin-density-wave (CDW/SDW) orders in superconducting cuprates has altered our perspective on the nature of high-temperature superconductivity (SC). However, it has proven difficult to fully elucidate the relationship between the density wave orders and SC. Here using resonant soft X-ray scattering we study the archetypal cuprate, La$_{2-x}$Sr$_x$CuO$_4$ (LSCO) over a broad doping range. We reveal the existence of two types of CDW orders in LSCO, namely CDW stripe order and CDW short-range order (SRO). While the CDW-SRO is suppressed by SC, it is partially transfor…
The effect of a magnetic field on the charge stripe order in La(2-x)Ba(x)CuO(4) has been studied by means of high energy (100 keV) x-ray diffraction for charge carrier concentrations ranging from strongly underdoped to optimally doped. We find that charge stripe order can be significantly enhanced by a magnetic field applied along the c-axis, but only at temperatures and dopings where it coexists with bulk superconductivity at zero field. The field also increases stripe correlations between the planes, which can result in an enhanced frustration of the interlayer Josephson coupling. Close to t…
The in-plane optical conductivity of seven La(2-x)Sr(x)CuO(4) single crystals with x between 0 and 0.15 has been studied from 30 to 295 K. All doped samples exhibit strong peaks in the far-infrared, which closely resemble those observed in Cu-O "ladders" with one-dimensional charge-ordering. The behavior with doping and temperature of the peak energy, width, and intensity allows us to conclude that we are observing charge stripes dynamics in La(2-x)Sr(x)CuO(4) on the fast time scale of infrared spectroscopy.
Random Fields from Quenched Disorder in an Archetype for Correlated Electrons: the Parallel Spin Stripe Phase of La$_{1.6-x}$Nd$_{0.4}$Sr$_x$CuO$_4$ at the 1/8 Anomaly
The interplay between charge order and superconductivity remains one of the central themes of research in quantum materials. In the case of cuprates, the coupling between striped charge fluctuations and local electromagnetic fields is especially important, as it affects transport properties, coherence and dimensionality of superconducting correlations. Here, we study the emission of coherent terahertz radiation in single-layer cuprates of the La$_{2-x}$Ba$_x$CuO$_4$ family, for which this effect is expected to be forbidden by symmetry. We find that emission vanishes for compounds in which the …
We demonstrate that the integrated intensity of Cu-63 nuclear quadrupole resonance (NQR) in La(1.6-x)Nd(0.4)Sr(x)CuO(4) decreases dramatically below the charge-stripe ordering temperature T(charge). Comparison with neutron and X-ray scattering indicates that the wipeout fraction F(T) (i.e. the missing fraction of the integrated intensity of the NQR signal) represents the charge-stripe order parameter. The systematic study reveals bulk charge-stripe order throughout the superconducting region 0.07 <= x <= 0.25. As a function of the reduced temperature t = T/T(charge), the temperature dependence…
Pulsed NQR at the frequencies of 28-33 MHz has been used to study copper NQR spectra in YBa{2}Cu{3}O{7}, TmBa{2}Cu{3}O{7} and Y{0.9}Pr{0.1}Ba{2}Cu{3}O{7} compounds at temperatures of 4.2-200K. Quantitative analysis of the spectra has shown that the "plane" Cu(2) spectra shape is well described by using a model of 1D correlations of charge and spin distribution in CuO{2} planes (stripe correlations). In the undoped superconductors the charge-spin stripe structure moves fast in the CuO{2} planes, but doping the YBa{2}Cu{3}O{7} lattice with praseodymium slows this motion down.
The Raman spectra on the cleaved surface of La$_{2-x}$Sr$_x$CuO$_4$ is found to be different from those on the mechanically polished or chemically etched surface. On the cleaved surface, the step-like increase of the scattering intensity below 700 cm$^{-1}$ is washed away and the two-phonon peaks are preserved clearly even at the optimum doping. The difference is demonstrated on the optimally doped crystal at x=0.15 and the stripe phase crystal at x=0.115. The stripe phase is stabilized by defects induced by mechanical polishing.
The evolution of an anelastic relaxation process occurring around 80 K in La{2-x}Sr{x}CuO{4} at a measuring frequency of ~1 kHz has been followed from x = 0.0075 to the overdoped region, x = 0.2, where it disappears. The dependence of the peak intensity on doping is consistent with a polaronic mechanism, identified with the disordered charge stripes overcoming pinning centers. A marked decrease of the peak amplitude occurs at x > 0.045, the same doping range where a change of the stripe order from parallel to diagonal with respect to the Cu-O bonds has been observed by neutron diffraction. Bot…
The correlations between stripe order, superconductivity, and crystal structure in La(2-x)Ba(x)CuO(4) single crystals have been studied by means of x-ray and neutron diffraction as well as static magnetization measurements. The derived phase diagram shows that charge stripe order (CO) coexists with bulk superconductivity in a broad range of doping around x=1/8, although the CO order parameter falls off quickly for x<>1/8. Except for x=0.155, the onset of CO always coincides with the transition between the orthorhombic and the tetragonal low temperature structures. The CO transition evolves fro…
We report an ultrahigh resolution resonant inelastic x-ray scattering (RIXS) study of the in-plane bond-stretching phonon mode in stripe-ordered cuprate La$_{1.675}$Eu$_{0.2}$Sr$_{0.125}$CuO$_4$. Phonon softening and lifetime shortening are found around the charge ordering wave vector. In addition to these self-energy effects, the electron-phonon coupling is probed by its proportionality to the RIXS cross section. We find an enhancement of the electron-phonon coupling around the charge-stripe ordering wave vector upon cooling into the low-temperature tetragonal structure phase. These results s…
This article presents the results of several magnetic phases of doped La$_{2-x}$Sr$_x$CuO$_4$ using density-functional theory with an added Hubbard term (DFT+U). Doping factors from $x=0$ to 0.25 were examined. We found that a bond centered stripe is the magnetic ground state for $x=1/8$ and $x=1/4$. No stable stripe order was found for $x=1/6$. Analysis of the electron density revealed that apical oxygen atoms, those located above and below the copper atoms in the CuO$_2$ planes, hold a non negligible part of the holes at large doping and present a small spin polarization. Finally, the charge…
Magnetic-field effects on the charge-spin stripe order in La-214 high-Tc cuprates have been investigated from measurements of the in-plane electrical-resistivity, Rho_ab_. In La_2-x_Ba_x_CuO_4_ with x=0.10 and La_2-x_Sr_x_CuO_4_ with x=0.115 where the incommensurate charge peaks are weak and unobservable in zero field in elastic neutron-scattering measurements, respectively, the normal-state value of Rho_ab_ at low temperatures markedly increases with increasing field up to 27 T. For La_2-x_Ba_x_CuO_4_ with x=0.11 and Zn-substituted La_2-x_Sr_x_Cu_1-y_Zn_y_O_4_ with x=0.115 and y=0.02 where th…
The relationships among charge order, spin fluctuations, and superconductivity in underdoped cuprates remain controversial. We use neutron scattering techniques to study these phenomena in La$_{1.93}$Sr$_{0.07}$CuO$_4$, a superconductor with a transition temperature of $T_c = 20$~K. At $T\ll T_c$, we find incommensurate spin fluctuations with a quasielastic energy spectrum and no sign of a gap within the energy range from 0.2 to 15 meV. A weak elastic magnetic component grows below $\sim10$~K, consistent with results from local probes. Regarding the atomic lattice, we have discovered unexpecte…
We measured reflectivity on static stripe-ordered La$_{1.84-y}$Nd$_y$Sr$_{0.16}$CuO$_4$ (LNSCO) $y$\,=\,0.1, 0.2, 0.3, and 0.4 by means of reflective terahertz time-domain spectroscopy (THz-TDS) with electric field polarized along c-axis, in which one can obtain lower frequency information than the conventional Fourier transform type spectrometer. Recently, two-dimensional superconducting (2DSC) property \cite{tajima,schafgans,li}, intra-layer perfect conductivity not accompanied with inter-layer superconducting behavior, was reported on LNSCO ($x$\,=0.15\,,\,$y$\,$\geq$\,0.2). We observed the…
We have studied the superexchange interaction $J_{ij}$ in doped $2D$ cuprates. The AFM interaction strongly depends on the state of the lattice of a CuO$_2$ layer surrounded by two LaO rock salt layers. In a static $U$ and $D$ stripe nanostructure, the homogeneous AFM interaction is impossible due to the $U/D/U...$ periodic stripe sequence and $T_N=0$. In a dynamic stripe nanostructure, the ideal CuO$_2$ layer with nonlocal effects and the homogeneous AFM interaction are restored. However the interaction $J_{ij}$ decreases by the exponential factor due to partial dynamic quenching. The meaning…
We report a detailed study of the temperature and magnetic-field dependence of the spin susceptibility for a single crystal of La(1.875)Ba(0.125)CuO(4). From a quantitative analysis, we find that the temperature-dependent anisotropy of the susceptibility, observed in both the paramagnetic and stripe-ordered phases, directly indicates that localized Cu moments dominate the magnetic response. A field-induced spin-flop transition provides further corroboration for the role of local moments. Contrary to previous analyses of data from polycrystalline samples, we find that a commonly-assumed isotrop…
Using polarized neutron scattering we establish that the magnetic order in La$_{1.48}$Nd$_{0.4}$Sr$_{0.12}$CuO$_4$ is either (i) one dimensionally modulated and collinear, consistent with the stripe model or (ii) two dimensionally modulated with a novel noncollinear structure. The measurements rule out a number of alternative models characterized by 2D electronic order or 1D helical spin order. The low-energy spin excitations are found to be primarily transversely polarized relative to the stripe ordered state, consistent with conventional spin waves.
We present and discuss the results of measurements of the ab-plane resistivity of La_{2-x}Sr_{x}CuO_{4} single crystals with small Sr contents (x=0.052-0.075). The resistivity was obtained in the temperature range between 4.2 K and 300 K by using an AC Van der Pauw technique. When the temperature is lowered, the rho_{ab}(T) curves show a transition from a linear behaviour to a semiconducting-like one. The deviation from the linearity occurs at a doping-dependent temperature T_{ch}. This effect can be interpreted as due to a progressive pinning of preexistent charge stripes. In the same framewo…
Quasi-two dimensional quantum magnetism is clearly highly correlated with superconducting ground states in cuprate-based High T$_c$ superconductivity. Three dimensional, commensurate long range magnetic order in La$_2$CuO$_4$ quickly evolves to quasi-two dimensional, incommensurate correlations on doping with mobile holes, and superconducting ground states follow for x as small as 0.05 in the La$_{2-x}$Sr$_x$/Ba$_x$CuO$_4$ family of superconductors. It has long been known that the onset of superconducting ground states in these systems is coincident with a remarkable rotation of the incommensu…
We report measurements of the longitudinal ($^{139}T_1^{-1}$) and transverse ($^{139}T_2^{-1}$) decay rates of the magnetization of $^{139}$La nuclei performed in a high quality single crystal of La$_{1.65}$Eu$_{0.2}$Sr$_{0.15}$CuO$_{4}$. We observe a dramatic slowing of the Cu 3d spins manifested as a sharp increase of both $^{139}T_1^{-1}$ and $^{139}T_2^{-1}$ below 30 K. We find that in this temperature range the fluctuations involve a unique time scale $τ$ which diverges as $(T-T_{\rm A})^{-1.9}$ with $T_{\rm A}\thickapprox 5$ K. This behavior is distinct from the continuous freezing obser…
We demonstrate that tunneling spectra in deeply underdoped Bi$_{2}$Sr$_{2}$CuO$_{6+δ}$ (Bi2201) and Ca$_2$CuO$_2$Cl$_2$ (CCOC) provide clear evidence for nanoscale phase separation (NPS), causing the gap to fill with doping rather than close. The phase separation extends over a doping range from half filling to approximately $x\sim 0.09$. Assuming the NPS is in the form of stripes, then the nodal gap -- which we model as a Coulomb gap -- arises from impurity pinning of the charged stripes, ultimately driving a metal-insulator transition.
The nature of charge stripe order and its relationship with structural phase transitions were studied using synchrotron X-ray diffraction in La$_{1.875}$Ba$_{0.125-x}$Sr$_{x}$CuO$_{4}$ ($0.05\leq x\leq 0.10$). For $x=0.05$, as temperature increased, incommensurate superlattice peaks associated with the charge order disappeared just at the structural phase transition temperature, $T_{\rm d2}$. However, for $x=0.075$ and 0.09, the superlattice peaks still existed as a short range correlation even above $T_{\rm d2}$, indicating a precursor of charge ordering. Furthermore, temperature dependences …
The charge and spin correlations in La$_{1.875}$Ba$_{0.125}$CuO$_4$ (LBCO 1/8) are studied using Cu $L_3$ edge resonant inelastic x-ray scattering (RIXS). The static charge order (CO) is observed at a wavevector of $(0.24,0)$ and its charge nature confirmed by measuring the dependence of this peak on the incident x-ray polarization. The paramagnon excitation in LBCO 1/8 is then measured as it disperses through the CO wavevector. Within the experimental uncertainty no changes are observed in the paramagnon due to the static CO, and the paramagnon seems to be similar to that measured in other cu…
Although all superconducting cuprates display charge-ordering tendencies, their low-temperature properties are distinct, impeding efforts to understand the phenomena within a single conceptual framework. While some systems exhibit stripes of charge and spin, with a locked periodicity, others host charge density waves (CDWs) without any obviously related spin order. Here we use resonant inelastic x-ray scattering (RIXS) to follow the evolution of charge correlations in the canonical stripe ordered cuprate La$_{1.875}$Ba$_{0.125}$CuO$_{4}$ (LBCO~$1/8$) across its ordering transition. We find tha…
High resolution angle-resolved photoemission measurements have been carried out on (La_1.4-xNd_0.6Sr_x)CuO_4, a model system with static stripes, and (La_1.85Sr_0.15)CuO_4, a high temperature superconductor (T_c=40K) with dynamic stripes. In addition to the straight segments near (pi, 0) and (0, pi) antinodal regions, we have identified the existence of nodal spectral weight and its associated Fermi surface in the electronic structure of both systems. The ARPES spectra in the nodal region show well-defined Fermi cut-off, indicating a metallic character of this charge-ordered state. This observ…
