Field-Controlled Magnetic Order in the Quantum Spin-Ladder System (Hpip)2CuBr4
B. Thielemann, Ch. Rüegg, K. Kiefer, H. M. Rønnow, B. Normand, P. Bouillot, C. Kollath, E. Orignac, R. Citro, T. Giamarchi, A. M. Läuchli, D. Biner, K. Krämer, … 展开作者
B. Thielemann, Ch. Rüegg, K. Kiefer, H. M. Rønnow, B. Normand, P. Bouillot, C. Kollath, E. Orignac, R. Citro, T. Giamarchi, A. M. Läuchli, D. Biner, K. Krämer, F. Wolff-Fabris, V. Zapf, M. Jaime, J. Stahn, N. B. Christensen, B. Grenier, D. F. McMorrow, J. Mesot
Neutron diffraction is used to investigate the field-induced, antiferromagnetically ordered state in the two-leg spin-ladder material (Hpip)2CuBr4. This "classical" phase, a consequence of weak interladder coupling, is nevertheless highly unconventional: its properties are influenced strongly by the spin Luttinger-liquid state of the ladder subunits. We determine directly the order parameter (transverse magnetization), the ordering temperature, the spin structure, and the critical exponents around the transition. We introduce a minimal, microscopic model for the interladder coupling and calculate the quantum fluctuation corrections to the mean-field interaction.
We present the results of muon-spin spectroscopy ($μ^{+}$SR) measurements on the molecular spin ladder system (Hpip)$_{2}$CuBr$_{4(1-x)}$Cl$_{4x}$, [Hpip=(C$_{5}$H$_{12}$N)]. Using transverse field $μ^{+}$SR we are able to identify characteristic behaviour in each of the regions of the phase diagram of the $x=0$ strong-rung spin ladder system (Hpip)$_{2}$CuBr$_4$. Comparison of our results to those of the dimer-based molecular magnet Cu(pyz)(gly)(ClO$_{4}$) shows several common features. We locate the crossovers in partially disordered (Hpip)$_{2}$CuBr$_{4(1-x)}$Cl$_{4x}$ ($x=0.05$), where a r…
Magnetic insulators have proven to be usable as quantum simulators for itinerant interacting quantum systems. In particular the compound (C$_{5}$H$_{12}$N)$_{2}$CuBr$_{4}$ (short (Hpip)$_{2}$CuBr$_{4}$) was shown to be a remarkable realization of a Tomonaga-Luttinger liquid (TLL) and allowed to quantitatively test the TLL theory. Substitution weakly disorders this class of compounds and allows thus to use them to tackle questions pertaining to the effect of disorder in TLL as well, such as the formation of the Bose glass. As a first step in this direction we present in this paper a study of th…
Analytic expressions for the correlation length temperature dependences are given for antiferromagnetic spin-1/2 Heisenberg ladders using a finite-size non-linear sigma-model approach. These calculations rely on identifying three successive crossover regimes as a function of temperature. In each of these regimes, precise and controlled approximations are formulated. The analytical results are found to be in excellent agreement with Monte Carlo simulations for the Heisenberg Hamiltonian.
In order to shed light whether the `even-odd conjecture' (even numbers of legs will superconduct accompanied by a spin gap while odd ones do not) for correlated electrons in ladder systems, the pairing correlation is studied for the Hubbard model on a two- and three-leg ladders. We have employed both the weak-coupling renormalization group and the quantum Monte Carlo (QMC) method for strong interactions. For the two-leg Hubbard ladder, a systematic QMC (with a controlled level spacings) has detected an enhanced pairing correlation, which is consistent with the weak-coupling prediction. We also…
Ultralow-Field Triplon Condensation in a Spin-Ladder Magnet
Charles University(查理大学);Technische Universität München(慕尼黑工业大学);VSB--Technical University of Ostrava(俄斯特拉发理工大学);University of Augsburg(奥格斯堡大学);CNRS, Université Grenoble Alpes(法国国家科学研究中心,格勒诺布尔阿尔卑斯大学);Rutherford Appleton Laboratory(鲁瑟福阿普尔顿实验室);Institut Laue-Langevin(朗之万研究所);European Spallation Source ERIC(欧洲散裂源)
One-magnon problem for spin-ladders with exact singlet-rung ground state in arbitrary oriented constant and staggered magnetic fields is studied. For two special configurations when the both fields are parallel or perpendicular to each other the exact formulas for eigenstates and eigenvectors are presented. In the parallel case the one-magnon contribution to the ESR absorption line shape is obtained. The latter is non-Lorentzian, has finite range and a gap around resonance. For low fields both the range of the spectrum and the width of the gap are controlled by the width of the one-magnon zone…
We present an extensive NMR study of the spin-1/2 antiferromagnetic Heisenberg ladder Cu2(C5H12N2)2Cl4 in a magnetic field range 4.5 - 16.7 T. By measuring the proton NMR relaxation rate 1/T_1 and varying the magnetic field around the critical field H_c1 = Delta / gμ_B = 7.5 T, we have studied the transition from a gapped spin liquid ground state to a gapless magnetic regime which can be described as a Luttinger liquid. We identify an intermediate regime T > |H-H_c1|, where the spin dynamics is (possibly) only controlled by the T=0 critical point H_c1.
Characterizing and accessing quantum phases of itinerant bosons or fermions in two dimensions (2D) that exhibit singular structure along surfaces in momentum space but have no quasi-particle description remains as a central challenge in the field of strongly correlated physics. Fortuitously, signatures of such 2D strongly correlated phases are expected to be manifest in quasi-one-dimensional "$N$-leg ladder" systems. The ladder discretization of the transverse momentum cuts through the 2D surface, leading to a quasi-1D descendant state with a set of low-energy modes whose number grows with the…
Controlled pairing symmetries in a Fermi-Hubbard ladder with band flattening
Centre for Quantum Optical Technologies, Centre of New Technologies, University of Warsaw(华沙大学新技术中心量子光学技术中心);Faculty of Physics, University of Warsaw(华沙大学物理学院);DIPC - Donostia International Physics Center(圣塞巴斯蒂安国际物理中心);Institute of Theoretical Physics, Wrocław University of Science and Technology(弗罗茨瓦夫科技大学理论物理研究所);Institute for Theoretical Physics, ETH Zürich(苏黎世联邦理工学院理论物理研究所);Max-Planck-Institut für Quantenoptik(马克斯·普朗克量子光学研究所);Munich Center for Quantum Science and Technology (MCQST)(慕尼黑量子科学与技术中心);Fakultät für Physik, Ludwig-Maximilians-Universität(路德维希-马克西米利安大学物理学院);ICFO-Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology(巴塞罗那科学与技术研究院光子科学研究所);IKERBASQUE, Basque Foundation for Science(伊克尔巴斯克,巴斯克科学基金会)
Stoner transitions beyond mean-field in two-dimensional electronic systems: a diagrammatic Monte Carlo study
School of Physics and Astronomy and William I. Fine Theoretical Physics Institute, University of Minnesota(明尼苏达大学物理与天文学学院及威廉·I·芬恩理论物理研究所);Department of Physics, University of Massachusetts, Amherst(马萨诸塞大学阿默斯特分校物理系)
Magnetic ground states of highly doped two-leg Hubbard ladders with a particle bath
Advanced Science Research Center, Japan Atomic Energy Agency(日本原子能机构先进科学研究中心);Department of Physics, Graduate School of Science, The University of Tokyo(东京大学理学研究科物理学系);JSR-UTokyo Collaboration Hub, CURIE(JSR-东京大学合作中心,CURIE)
The enigmatic scaling behaviour of the normal state properties of the high Tc cuprates has been explained by assuming that a crossover from the two- dimensional Heisenberg (2D-H) to the one-dimensional spin ladder (1D-SL) regime takes place at temperature T=T*. For T<T* stripe formation results in the quantum 1D transport with the characteristic inelastic length L_phi being fully controlled by the magnetic correlation length xi_m of the even-chain SL, whereas for T> T* the 2D quantum transport is realized with L_ϕgoverned by the 2D-H correlations L_phi=xi_m=exp(J/T)$. Therefore, the pseudogap …
The ordered hexagonal perovskite Ba2CuTeO6 hosts weakly coupled S=1/2 spin ladders produced by an orbital ordering of Cu2+. The magnetic susceptibility chi(T) of Ba2CuTeO6 is well described by that expected for isolated spin ladders with exchange coupling of J~86 K but shows a deviation from the expected thermally activated behavior at low temperatures below T*~25 K. An anomaly in chi(T), indicative of magnetic ordering, is observed at T_mag=16 K. No clear signature of long-range ordering, however, is captured in NMR, specific heat or neutron diffraction measurements at and below T_mag. The ma…
Condensed matter physics of gauge theories coupled to fermions can exhibit a rich phase structure, but are nevertheless very difficult to study in Monte Carlo simulations when they are afflicted by a sign problem. As an alternate approach, we use tensor network methods to explore the finite density physics of Abelian gauge theories without dynamical matter. As a concrete example, we consider the U(1) gauge invariant quantum link ladder with spin-1/2 gauge fields in an external electric field which cause the winding electric fluxes to condense in the ground state. We demonstrate how the electri…
Developing a theoretical framework to access quantum phases of itinerant bosons or fermions in two dimensions (2D) that exhibit singular structure along surfaces in momentum space but have no quasi-particle description remains as a central challenge in the field of strongly correlated physics. In this paper we propose that distinctive signatures of such 2D strongly correlated phases will be manifest in quasi-one-dimensional "N-leg ladder" systems. Characteristic of each parent 2D quantum liquid would be a precise pattern of 1D gapless modes on the N-leg ladder. These signatures could be potent…
The quest for experimental platforms that allow for the exploration, and even control, of the interplay of low dimensionality and frustration is a fundamental challenge in several fields of quantum many-body physics, such as quantum magnetism. Here, we propose the use of cold crystals of trapped ions to study a variety of frustrated quantum spin ladders. By optimizing the trap geometry, we show how to tailor the low dimensionality of the models by changing the number of legs of the ladders. Combined with a method for selectively hiding of ions provided by laser addressing, it becomes possible …
Identification and optimization of accurate spin models for Fermi-Hubbard ladders using matrix product states
Donostia International Physics Center (DIPC)(多诺斯蒂亚国际物理中心);University of the Basque Country (UPV/EHU)(巴斯克大学);IKERBASQUE, Basque Foundation for Science(伊克尔巴斯基奎,巴斯克科学基金会)
Numerical studies of the reduced density matrix of a gapped spin-1/2 Heisenberg antiferromagnet on a two-leg ladder find that it has the same form as the Gibbs density matrix of a gapless spin-1/2 Heisenberg antiferromagnetic chain at a finite temperature determined by the spin gap of the ladder. We investigate this interesting result by considering a model of free fermions on a two-leg ladder (gapped by the inter-chain tunneling operator) and in spin systems on a ladder with a gapped ground state using exact solutions and several controlled approximations. We calculate the reduced density mat…
In most lattice models, the closing of a band gap typically occurs at high-symmetry points in the Brillouin zone. Differently, in the Creutz model $-$ describing a system of spinless fermions hopping on a two-leg ladder pierced by a magnetic field $-$ the gap closing at the quantum phase transition between the two topologically nontrivial phases of the model can be moved by tuning the hopping amplitudes. We take advantage of this property to examine the nonequilibrium dynamics of the model after a sudden quench of the magnetic flux through the plaquettes of the ladder. For a quench to one of t…
Classical and quantum phase transitions (QPTs), with their accompanying concepts of criticality and universality, are a cornerstone of statistical thermodynamics. An exemplary controlled QPT is the field-induced magnetic ordering of a gapped quantum magnet. Although numerous "quasi-one-dimensional" coupled spin-chain and -ladder materials are known whose ordering transition is three-dimensional (3D), quasi-2D systems are special for several physical reasons. Motivated by the ancient pigment Han Purple (BaCuSi$_{2}$O$_{6}$), a quasi-2D material displaying anomalous critical properties, we prese…
We propose an unconventional topological quantum phase transition connecting a higher-order topological insulator (HOTI) and a featureless Mott insulator sharing the same symmetry patterns. We construct an effective theory description of the quantum critical point (QCP) by combining a bosonization approach and the coupled-stripe construction of 1D critical spin ladders. The phase transition theory is characterized by a critical dipole liquid theory with subsystem $U(1)$ symmetry whose low energy modes contain a Bose surface along the $k_x,k_y$ axis. Such a quantum critical point manifests frac…
The quantum spin systems Cu$_2$M'BO$_5$ (M' = Al, Ga) with the ludwigite crystal structure consist of a structurally ordered Cu$^{2+}$ sublattice in the form of three-leg ladders, interpenetrated by a structurally disordered sublattice with a statistically random site occupation by magnetic Cu$^{2+}$ and nonmagnetic Ga$^{3+}$ or Al$^{3+}$ ions. A microscopic analysis based on density-functional-theory calculations for Cu$_2$GaBO$_5$ reveals a frustrated quasi-two-dimensional spin model featuring five inequivalent antiferromagnetic exchanges. A broad low-temperature $^{11}$B nuclear magnetic re…