Ivan C. H. Liu, Jovica Stanojevic, Jan M. Rost
A Rydberg and a ground-state atom can form ultralong range diatomic molecules provided the interaction between the ground-state atom and the Rydberg electron is attractive [C. H. Greene, et al., Phys. Rev. Lett. 85, 2458 (2000)]. A repulsive interaction does not support bound states. However, as we will show, adding a second ground-state atom, a bound triatomic molecule becomes possible constituting a Borromean Rydberg system.
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Ultralong-range Rydberg trimer molecules are spectroscopically observed in an ultracold gas of Cs($nd_{3/2}$) atoms. The atomic Rydberg state anisotropy allows for the formation of angular trimer states, whose energies may not be obtained from integer multiples of dimer energies. These nonadditive trimers are predicted to coexist with Rydberg dimer lines. The existence of such effective three-body interactions is confirmed with observation of asymmetric line profiles and interpreted by a theoretical approach which includes relativistic spin interactions. Simulations of the observed spectra wit…
Effects of $p$-wave Interactions on Borromean Efimov Trimers in Heavy-Light Fermi Systems
本文研究质量比大于13.6的重-轻费米系统中$p$波相互作用对Borromean Efimov三聚体的影响，发现$p$波费米子-费米子相互作用会破坏临界$s$波散射长度的普适性并有利于Borromean态形成，且Efimov效应在$p$波幺正极限下依然存在。
Three-body Förster resonances at long-range interactions of Rydberg atoms were first predicted and observed in Cs Rydberg atoms by R.Faoro et al., Nature Comm. 6, 8173 (2015). In these resonances, one of the atoms carries away an energy excess preventing the two-body resonance, leading thus to a Borromean type of Förster energy transfer. But they were in fact observed as the average signal for the large number of atoms $N\gg1$. In this Letter we report on the first experimental observation of the three-body Förster resonances ${\rm 3}\times nP_{3/2} (|{\rm M}|)\to nS_{1/2} +(n+1)S_{1/2} +nP_{3…
We have observed recently the Stark-tuned three-body Förster resonances ${\rm 3}\times nP_{3/2} (|M|)\to nS_{1/2} +(n+1)S_{1/2} +nP_{3/2} (|M^{*} |)$ at long-range interactions of a few cold Rb Rydberg atoms [D.B.Tretyakov et al., Phys. Rev. Lett. 119, 173402 (2017)]. The three-body resonance appears at a different dc electric field with respect to the ordinary two-body resonance ${\rm 2}\times nP_{3/2} (|M|)\to nS_{1/2} +(n+1)S_{1/2} $ and corresponds to a transition when the three interacting atoms change their states simultaneously (two atoms go to the $S$ states, and the third atom remains…
Ultracold long-range van der Waals Rydberg trimer
本研究预测稀薄原子-气体混合物中存在由里德伯原子与双原子极性分子构成的超长程范德瓦尔斯三聚物，给出其尺寸、结合能及双光子光缔合产生速率，并论证共振观测可行性。
We measure nonlocal third-order spatial correlations in non-degenerate ultracold gases of bosonic ($^{84}$Sr) and spin-polarized fermionic ($^{87}$Sr) strontium through studies of the formation rates for ultralong-range trimer Rydberg molecules. The trimer production rate is observed to be very sensitive to the effects of quantum statistics with a strong enhancement of up to a factor of six (3!) in the case of bosonic $^{84}$Sr due to bunching, and a marked reduction for spin-polarized fermionic $^{87}$Sr due to anti-bunching. The experimental results are compared to theoretical predictions an…
We show that the recently observed class of long-range ion-Rydberg molecules can be divided into two families of states, which are characterised by their unique electronic structures resulting from the ion-induced admixture of quantum defect-split Rydberg $n$P states with different low-field seeking high-$l$ states. We predict that in both cases these diatomic molecular states can bind additional ground state atoms lying within the orbit of the Rydberg electron, thereby forming charged ultralong-range Rydberg molecules (ULRM) with binding energies similar to that of conventional non-polar ULRM…
Quantum reflection is a pure wave phenomena that predicts reflection of a particle at a changing potential for cases where complete transmission occurs classically. For a chemical bond, we find that this effect can lead to non-classical vibrational turning points and bound states at extremely large interatomic distances. Only recently has the existence of such ultralong-range Rydberg molecules been demonstrated experimentally. Here, we identify a broad range of molecular lines, most of which are shown to originate from two different novel sources: a single-photon associated triatomic molecule …
We show that the dipole-dipole interaction between three identical Rydberg atoms can give rise to bound trimer states. The microscopic origin of these states is fundamentally different from Efimov physics. Two stable trimer configurations exist where the atoms form the vertices of an equilateral triangle in a plane perpendicular to a static electric field. The triangle edge length typically exceeds $R\approx 2\,μ\text{m}$, and each configuration is two-fold degenerate due to Kramers' degeneracy. The depth of the potential wells and the triangle edge length can be controlled by external paramet…
We study ultracold long-range collisions of heteronuclear alkali-metal dimers with a reservoir gas of alkali-metal Rydberg atoms in a two-photon laser excitation scheme. In a low density regime where molecules remain outside the Rydberg orbits of the reservoir atoms, we show that the two-photon photoassociation (PA) of the atom-molecule pair into a long-range bound trimer state is efficient over a broad range of atomic Rydberg channels. As a case study, we obtain the PA lineshapes for the formation of trimers composed of KRb molecules in the rovibrational ground state and excited Rb atoms in t…
We show that the resonant dipole-dipole interaction can give rise to bound states between two and three Rydberg atoms with non-overlapping electron clouds. The dimer and trimer states arise from avoided level crossings between states converging to different fine structure manifolds in the limit of separated atoms. We analyze the angular dependence of the potential wells, characterize the quantum dynamics in these potentials and discuss methods for their production and detection. Typical distances between the atoms are of the order of several micrometers which can be resolved in state-of-the-ar…
Metastable doubly-charged Rydberg molecules
本文预测了由$^{87}$Rb里德堡原子与一对阳离子构成的长程三聚体$^{87}$Rb$_3^{2+}$存在亚稳态振动束缚态，其束缚源于离子与里德堡原子四极矩的相互作用，且稳定性对主量子数高度敏感。
We investigate triatomic molecules that consist of two ground state atoms and a highly excited Rydberg atom, bound at large internuclear distances of thousands of Ångstroms. In the molecular state the Rydberg electron is in a superposition of high angular momentum states whose probability densities resemble the form of trilobite fossils. The associated potential energy landscape has an oscillatory shape and supports a rich variety of stable geometries with different bond angles and bond lengths. Based on an electronic structure investigation we analyze the molecular geometry systematically and…
Ground-state phase diagram of Rydberg atoms in a triangular-prism array
利用密度矩阵重正化群研究三角棱柱光镊阵列中里德伯原子的基态相图，通过调节失谐-拉比频率比和里德伯阻塞半径，发现了多种密度波相及其相变，包括Z2平移对称性破缺、D3对称性破缺以及丰富的临界行为。
We find that energy surfaces of more than two atoms or molecules interacting via dipole-dipole po- tentials generically possess conical intersections (CIs). Typically only few atoms participate strongly in such an intersection. For the fundamental case, a circular trimer, we show how the CI affects adiabatic excitation transport via electronic decoherence or geometric phase interference. These phe- nomena may be experimentally accessible if the trimer is realized by light alkali atoms in a ring trap, whose dipole-dipole interactions are induced by off-resonant dressing with Rydberg states. Suc…
Rubidium Rydberg atoms in either $|m_j|$-sublevel of the $36p_{3/2}$ state can exchange energy via Stark-tuned Förster resonances, including two-, three-, and four-body dipole-dipole interactions. Three-body interactions of this type were first reported and categorized by Faoro, \textit{et al.}~[Nat.\ Commun.\ \textbf{6}, 8173 (2015)] and their Borromean nature was confirmed by Tretyakov, \textit{et al.}~[Phys.\ Rev.\ Lett. \textbf{119}, 173402 (2017)]. We report the time dependence of the $N$-body Förster resonance $N\times 36p_{3/2,|m_j|=1/2}\rightarrow 36s_{1/2}+37s_{1/2}+(N-2)\times 36p_{3…
We detail the rich electronic and vibrational structure of triatomic "butterfly" molecules, ultra-long-range Rydberg molecules bound by resonant $p$-wave scattering. We divide these molecules into two sub-classes depending on their parity under reflection of the electronic wave function through the molecular plane. The trimers with odd reflection parity have topographically smooth potential energy surfaces except near the collinear configuration. Here, the vibrational wave function is confined tightly in the symmetric-stretch and bending modes, but only loosely in the asymmetric stretch mode. …
We report spectroscopic observation of Rydberg polarons in an atomic Bose gas. Polarons are created by excitation of Rydberg atoms as impurities in a strontium Bose-Einstein condensate. They are distinguished from previously studied polarons by macroscopic occupation of bound molecular states that arise from scattering of the weakly bound Rydberg electron from ground-state atoms. The absence of a $p$-wave resonance in the low-energy electron-atom scattering in Sr introduces a universal behavior in the Rydberg spectral lineshape and in scaling of the spectral width (narrowing) with the Rydberg …
Topological edge states in a Rydberg composite
本研究聚焦里德堡复合物的拓扑相问题，通过其电子哈密顿量与紧束缚模型的映射，证实了拓扑保护边缘态的存在，并拓展了三聚体元胞等复杂拓扑体系的模拟途径。
Feshbach resonances in ultra-cold atomic gases have led to some of the most important advances in atomic physics. They did not only enable ground breaking work in the BEC-BCS crossover regime [1], but are also widely used for the association of ultra-cold molecules [2], leading to the formation of molecular Bose-Einstein condensates [3,4] and ultra-cold dipolar molecular systems [5]. Here, we demonstrate the experimental realization of an optical Feshbach resonance using ultra-long range Rydberg molecules [6]. We show their practical use by tuning the revival time of a quantum many-body system…
Bound states of massive particles, such as nuclei, atoms or molecules, constitute the bulk of the visible world around us. In contrast, photons typically only interact weakly. We report the observation of traveling three-photon bound states in a quantum nonlinear medium where the interactions between photons are mediated by atomic Rydberg states. Photon correlation and conditional phase measurements reveal the distinct bunching and phase features associated with three-photon and two-photon bound states. Such photonic trimers and dimers possess shape-preserving wavefunctions that depend on the …
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