We demonstrate experimentally manipulation of supercurrent in Al-AlO_x-Ti Josephson tunnel junctions by injecting quasiparticles in a Ti island from two additional tunnel-coupled Al superconducting reservoirs. Both supercurrent enhancement and quenching with respect to equilibrium are achieved. We demonstrate cooling of the Ti line by quasiparticle injection from the normal state deep into the superconducting phase. A model based on heat transport and non-monotonic current-voltage characteristic of a Josephson junction satisfactorily accounts for our findings.
We report on the fabrication and characterization of a two-terminal mesoscopic interferometer based on three V/Cu/V Josephson junctions having nanoscale cross-section. The junctions have been arranged in a double-ring geometry realized by metallic thin film deposition through a suspended mask defined by electron beam lithography. Although a significant amount of asymmetry between the critical current of each junction is observed we show that the interferometer is able to suppress the supercurrent to a level lower than 6 parts per thousand, being here limited by measurement resolution. The pres…
In this paper we address several new developments in the theory of dc Josephson effect in superconducting weak links. We analyze an interplay between quantum interference effects and Andreev reflection in SNS nanojunctions with insulating barriers and demonstrate that such effects may qualitatively modify the Josephson current in such structures. We also investigate an impact of the parity effect on persistent currents in superconducting nanorings interrupted by a quantum point contact (QPC). In the limit of zero temperature and for the odd number of electrons in the ring we predict complete s…
Utilizing a full microscopic Bogoliubov-de Gennes (BdG) approach, we study the equilibrium charge and spin currents in ballistic $SFSFS$ Josephson systems, where $F$ is a uniformly magnetized ferromagnet and $S$ is a conventional $s$-wave superconductor. From the spatially varying spin currents, we also calculate the associated equilibrium spin transfer torques. Through variations in the relative phase differences between the three $S$ regions, and magnetization orientations of the ferromagnets, our study demonstrates tunability and controllability of the spin and charge supercurrents. The spi…
The multi-terminal Josephson effect allows DC supercurrent to flow at finite commensurate voltages. Existing proposals to realize this effect rely on nonlocal Andreev processes in superconductor-normal-superconductor junctions. However, this approach requires precise control over microscopic states and is obscured by dissipative current. We show that standard tunnel Josephson circuits also support multiplet supercurrent mediated only by local tunneling processes. Furtheremore, we observe that the supercurrents persist even in the high charging energy regime in which only sequential Cooper tran…
We apply the mechanically controllable break junctions technique to investigate the transition from tunneling to direct contact in tungsten. This transition is quite different from that of other metals and is determined by the local electronic properties of the tungsten surface and the relief of the electrodes at the point of their closest proximity. The conductance traces show a rich variety of patterns from the avalanche-like jump to a mesoscopic contact to the completely smooth transition between direct contact and tunneling. Due to the occasional absence of an adhesive jump the conductance…
We theoretically investigate heat transport in hybrid normal metal-superconductor (NS) nanojunctions focusing on the effect of thermal rectification. We show that the heat diode effect in the junction strongly depends on the transmissivity and the nature of the NS contact. Thermal rectification efficiency can reach up to 123% for a fully-transmissive ballistic junction and up to 84% in diffusive NS contacts. Both values exceed the rectification efficiency of a NIS tunnel junction (I stands for an insulator) by a factor close to 5 and 3, respectively. Furthermore, we show that for NS point-cont…
We study the interaction between single apex atoms in a metallic contact, using the break junction geometry. By carefully 'training' our samples, we create stable junctions in which no further atomic reorganization takes place. This allows us to study the relation between the so-called jump out of contact (from contact to tunnelling regime) and jump to contact (from tunnelling to contact regime) in detail. Our data can be fully understood within a relatively simple elastic model, where the elasticity k of the electrodes is the only free parameter. We find 5 < k < 32 N/m. Furthermore, the inter…
We study the tunneling transport through a nanojunction in the far-from-equilibrium regime at relatively low temperatures. We show that the current-voltage characteristics is significantly modified as compared to the usual quasi-equilibrium result by lifting the suppression due to the Coulomb blockade. These effects are important in realistic nanojunctions. We study the high-impedance case in detail to explain the underlying physics and construct a more realistic theoretical model for the case of a metallic junction taking into account dynamic Coulomb interaction. This dynamic screening furthe…
When two superconductors become electrically connected by a weak link a zero-resistance supercurrent can flow. This supercurrent is carried by Cooper pairs of electrons with a combined charge of twice the elementary charge, e. The 2e charge quantum is clearly visible in the height of Shapiro steps in Josephson junctions under microwave irradiation and in the magnetic flux periodicity of h/2e in superconducting quantum interference devices. Several different materials have been used to weakly couple superconductors, such as tunnel barriers, normal metals, or semiconductors. Here, we study super…
We show that in the presence of ferromagnetic electronic reservoirs and spin-dependent tunnel couplings, molecular vibrations in nonmagnetic single molecular transistors induce an effective intramolecular exchange magnetic field. It generates a finite spin-accumulation and -precession for the electrons confined on the molecular bridge and occurs under (non)equilibrium conditions. The effective exchange magnetic field is calculated here to lowest order in the tunnel coupling for a nonequilibrium transport setup. Coulomb interaction between electrons is taken into account as well as a finite ele…
A Kapitza Pendulum Route to Supercurrent Tunnel Diodes
Istituto di Struttura della Materia of the National Research Council（国家研究委员会材料结构研究所）；Institute for Theoretical Solid State Physics, IFW Dresden（德累斯顿IFW理论固体质物理研究所）；CNR-SPIN；Istituto Lombardo “Accademia di Scienze e Lettere”（伦巴第科学院与文学院）；NEST Istituto Nanoscienze-CNR and Scuola Normale Superiore（CNR纳米科学研究所NEST与比萨高等师范学院）；Würzburg-Dresden Cluster of Excellence ct.qmat（维尔茨堡-德累斯顿卓越集群ct.qmat）；Universitá di Salerno（萨莱诺大学）
Graphene electrodes provide a suitable alternative to metal contacts in molecular conduction nanojunctions. Here, we propose to use graphene electrodes as a platform for effective photon assisted tunneling through molecular conduction nanojunctions. We predict dramatic increasing currents evaluated at side-band energies $\sim n\hbarω$ ($n$ is a whole number) related to the modification of graphene gapless spectrum under the action of external electromagnetic field of frequency $ω$. A side benifit of using doped graphene electrodes is the polarization control of photocurrent related to the proc…
We study the Josephson effect for a topologically nontrivial superconducting (TS) wire with Majorana fermion end states and tunnel-coupled to s-wave BCS superconducting (S) electrodes. In an S-TS junction, no supercurrent flow is possible under fairly general conditions. For the S-TS-S junction, bulk TS quasiparticles must be accessible to have a Josephson effect. In the noninteracting case, we derive the exact current-phase relation (CPR) and find π-periodic behavior with negative critical current for weak tunnel couplings. Charging effects then cause the anomalous CPR $I(φ)=I_c \cosφ$, where…
Efficient operation of electronic nanodevices at ultrafast speeds requires understanding and control of the currents generated by femtosecond bursts of light. Ultrafast laser-induced currents in metallic nanojunctions can originate from photo-assisted hot electron tunneling or lightwave-induced tunneling. Both processes can drive localized photocurrents inside a scanning tunneling microscope (STM) on femto- to attosecond time scales, enabling ultrafast STM with atomic spatial resolution. Femtosecond laser excitation of a metallic nanojunction, however, also leads to the formation of a transien…
Noise measurements are a probe beyond simple electronic transport that can reveal additional information about electronic correlations and inelastic processes. Here we report noise measurements in individual electromigrated nanojunctions, examining the evolution from the many channel regime to the tunneling regime, using a radio frequency technique. While we generally observe the dependence of noise on bias expected for shot noise, in approximately 12% of junction configurations we find discrete changes in the bias dependence at threshold values of the bias, consistent with electronic excitati…
Understanding the process of electron tunneling in chirality-induced single-molecule junctions is imperative for the development of nanoscale switching and artificial nanomotors. Based on the combined non-equilibrium Green functions formalism and the ground-state density functional theory, we present here the charge transport behavior of chiral gold (7,3) nanowires (NWs) in comparison with various other chiral and achiral 1D gold nanostructures as the principal leads to form stable single-molecule junctions. For sigma-saturated alkane chains, we find that the contact potential barriers vary wi…
Using tunneling spectroscopy, we have measured the local electron energy distribution function in the normal part of a superconductor-normal metal-superconductor (SNS) Josephson junction containing an extra lead to a normal reservoir. In the presence of simultaneous supercurrent and injected quasiparticle current, the distribution function exhibits a sharp feature at very low energy. The feature is odd in energy, and odd under reversal of either the supercurrent or the quasiparticle current direction. The feature represents an effective temperature gradient across the SNS Josephson junction th…
A nondissipative supercurrent state of a Josephson junction is metastable with respect to the formation of a finite-resistance state. This transition is driven by fluctuations, thermal at high temperatures and quantum at low temperatures. We evaluate the life time of such a state due to quantum fluctuations in the limit when the supercurrent is approaching the critical current. The decay probability is determined by the instanton action for the superconducting phase difference across the junction. At low temperatures, dynamics of the phase is massive and is determined by the effective capacita…
The RCSJ model of resistively and capacitively shunted Josephson junctions is used to describe superconducting point contacts over a wide range of resistances up to the metallic -- tunneling transition. Their small dynamic capacitance of order $C = 0.1 $fF due to the point-contact geometry results in a huge plasma frequency. The critical current is then strongly suppressed and the contact resistance becomes finite because of quantum-mechanical zero-point fluctuations of the Josephson plasma and the rather large escape rate out of the zero-voltage state due to quantum tunneling. We test the pre…
We study the nonequilibrium characteristics of superconducting tunnel structures in the case when one of the superconductors is a small island confined between large superconductors. The state of this island can be probed for example via the supercurrent flowing through it. We study both the far-from-equilibrium limit when the rate of injection for the electrons into the island exceeds the energy relaxation inside it, and the quasiequilibrium limit when the electrons equilibrate between themselves. We also address the crossover between these limits employing the collision integral derived for …
We study a two-terminal graphene Josephson junction with contacts shaped to form a narrow constriction, less than 100nm in length. The contacts are made from type II superconducting contacts and able to withstand magnetic fields high enough to reach the quantum Hall (QH) regime in graphene. In this regime, the device conductance is determined by edge states, plus the contribution from the constricted region. In particular, the constriction area can support supercurrents up to fields of ~2.5T. Moreover, enhanced conductance is observed through a wide range of magnetic fields and gate voltages. …
Electronic transport through nanostructures is greatly affected by the presence of superconducting leads. If the interface between the nanostructure and the superconductors is sufficiently transparent, a dissipationless current (supercurrent) can flow through the device due to the Josephson effect. A Josephson coupling, as measured via the zero-resistance supercurrent, has been obtained via tunnel barriers, superconducting constrictions, normal metals, and semiconductors. The coupling mechanisms vary from tunneling to Andreev reflection. The latter process has always occurred via a normal-type…
We study a Cooper-pair transistor realized by two Josephson weak links that enclose a superconducting island in an InSb-Al hybrid nanowire. When the nanowire is subject to a magnetic field, isolated subgap levels arise in the superconducting island and, due to the Coulomb blockade,mediate a supercurrent by coherent co-tunneling of Cooper pairs. We show that the supercurrent resulting from such co-tunneling events exhibits, for low to moderate magnetic fields, a phase offset that discriminates even and odd charge ground states on the superconducting island. Notably,this phase offset persists wh…
We study mesoscopic fluctuations and weak localization correction to the supercurrent in Josephson junctions with coherent diffusive electron dynamics in the normal part. Two kinds of junctions are considered: a chaotic dot coupled to superconductors by tunnel barriers and a diffusive junction with transparent normal--superconducting interfaces. The amplitude of current fluctuations and the weak localization correction to the average current are calculated as functions of the ratio between the superconducting gap and the electron dwell energy, temperature, and superconducting phase difference …
A Josephson tunnel junction transistor based on quasiparticle injection is proposed. Its operation relies on the manipulation of the electron distribution in one of the junction electrodes. This is accomplished by injecting quasiparticle current through the junction electrode by two additional tunnel coupled superconductors. Both large supercurrent enhancement and fast quenching can be achieved with respect to equilibrium by varying quasiparticle injection for proper temperature regimes and suitable superconductor combinations. Joined with large power gain this makes the device attractive for …
We propose a model for resonant Josephson tunneling through quantum dots that accounts for Cooper pair-breaking processes in the superconducting leads caused by a magnetic field or spin-flip scattering. The pair-breaking effect on the critical supercurrent $I_c$ and the Josephson current-phase relation $I(ϕ)$ is largely due to the modification of the spectrum of Andreev bound states below the reduced (Abrikosov-Gorkov) quasiparticle gap. For a quantum dot formed in a quasi-one-dimensional channel, both $I_c$ and $I(ϕ)$ can show a significant magnetic field dependence induced by pair breaking d…
Recent advances have attracted attention to non-standard Josephson junctions in which a supercurrent can flow despite zero phase difference between the constituent superconducting leads. Here, we propose a zero-phase-difference nanoelectromechanical junction which, in contrast to other considered systems, exhibits symmetry between leftward and rightward tunneling through the junction. We show that a supercurrent is nevertheless possible as a result of spontaneous symmetry breaking. In the suggested junction, the supercurrent is mediated by tunneling via a superconducting Cooper-pair box on a b…
Using the Keldysh-Usadel formalism, we theoretically study the $0$-$π$ transition profiles and current-phase relations of magnetic $SFSFS$ and $SFSFFS$ Josephson nanojunctions in the diffusive regime. By allowing the magnetizations of the ferromagnetic layers to take arbitrary orientations, the strength and direction of the charge supercurrent flowing through the ferromagnetic regions can be controlled via the magnetization rotation in one of the ferromagnetic layers. Depending on the junction parameters, we find opposite current flow in the ferromagnetic layers, revealing that remarkably such…
The dc Josephson effect in a superconducting quantum point contact, where supercurrent flows through a small number of channels, is reviewd. The central role of Andreev levels is emphasized which carry the whole supercurrent in short symmetric Josephson junctions including tunnel junctions. A simple intuitive view of the dc Josephson effect in a quantum point contact is given in terms of multiple Andreev reflections. The quantization of the critical current in superconducting quantum point contacts is briefly discussed.
In the classical Josephson effect the phase difference across the junction is well defined, and the supercurrent is reduced only weakly by phase diffusion. For mesoscopic junctions with small capacitance the phase undergoes large quantum fluctuations, and the current is also decreased by Coulomb blockade effects. We discuss the behavior of the current-voltage characteristics in a large range of parameters comprising the phase diffusion regime with coherent Josephson current as well as the supercurrent peak due to incoherent Cooper pair tunneling in the Coulomb blockade regime.
We investigate the quantum heat exchange between a nanojunction and a many-body or electromagnetic environment far from equilibrium. It is shown that the two-temperature energy emission-absorption mechanism gives rise to a giant heat flow between the junction and the environment. We obtain analytical results for the heat flow in an idealized high impedance environment and perform numerical calculations for the general case of interacting electrons and discuss the giant freezing and heating effects in the junction under typical experimental conditions.
Local spins coupled to superconductors give rise to several emerging phenomena directly linked to the competition between Cooper pair formation and magnetic exchange. These effects are generally scrutinized using a spectroscopic approach which relies on detecting the in-gap bound modes arising from Cooper pair breaking, the so-called Yu-Shiba-Rusinov (YSR) states. However, the impact of local magnetic impurities on the superconducting order parameter remains largely unexplored. Here, we use scanning Josephson spectroscopy to directly visualize the effect of magnetic perturbations on Cooper pai…
Supercurrent detection and manipulation of topological phase transitions in Shiba-Majorana hybrid systems
Physical Research Laboratory（物理研究实验室）；Technische Universität Braunschweig（布伦瑞克工业大学）；The Hamburg Centre for Ultrafast Imaging（汉堡超快成像中心）；Universität Hamburg（汉堡大学）；International Research Centre MagTop, Institute of Physics, Polish Academy of Sciences（波兰科学院物理研究所磁拓扑国际研究中心）；University of Basel（巴塞尔大学）
The supercurrent of a Josephson junction is reduced by phase diffusion. For ultrasmall capacitance junctions the current may be further decreased by Coulomb blockade effects. We calculate the Cooper pair current by means of time-dependent perturbation theory to all orders in the Josephson coupling energy and obtain the current-voltage characteristic in closed form in a range of parameters of experimental interest. The results comprehend phase diffusion of the coherent Josephson current in the classical regime as well as the supercurrent peak due to incoherent Cooper pair tunneling in the stron…
An interlayer phase coherence develops spontaneously in the bilayer quantum Hall system at the filling factor $ν=1$. On the other hand, the spin and pseudospin degrees of freedom are entangled coherently in the canted antiferromagnetic phase of the bilayer quantum Hall system at the filling factor $ν=2$. There emerges a complex Nambu-Goldstone mode with a linear dispersion in the zero tunneling-interaction limit for both cases. Then its phase field provokes a Josephson supercurrent in each layer, which is dissipationless as in a superconductor. We study what kind of phase coherence the Nambu-G…
We present a theory of transport through interacting quantum dots coupled to normal and superconducting leads in the limit of weak tunnel coupling. A Josephson current between two superconducting leads, carried by first-order tunnel processes, can be established by non-equilibrium proximity effect. Both Andreev and Josephson current is suppressed for bias voltages below a threshold set by the Coulomb charging energy. A $π$-transition of the supercurrent can be driven by tuning gate or bias voltages.
We have developed a quantitative theory of Cooper pair pumping in gated one-dimensional arrays of Josephson junctions. The pumping accuracy is limited by quantum tunneling of Cooper pairs out of the propagating potential well and by direct supercurrent flow through the array. Both corrections decrease exponentially with the number N of junctions in the array, but give a serious limitation of accuracy for any practical array. The supercurrent at resonant gate voltages decreases with N only as sin(v/N)/N, where v is the Josephson phase difference across the array.
We consider a combined nanomechanical-supercondcuting device that allows the Cooper pair tunneling to interfere with the mechanical motion of the middle superconducting island. Coupling of mechanical oscillations of a superconducting island between two superconducting leads to the electronic tunneling generate a supercurrent which is modulated by the oscillatory motion of the island. This coupling produces alternating finite and vanishing supercurrent as function of the superconducting phases. Current peaks are sensitive to the superconducting phase shifts relative to each other. The proposed …
We measure the non-dissipative supercurrent in a single InAs self-assembled quantum dot (QD) coupled to superconducting leads. The QD occupation is both tuned by a back-gate electrode and lateral side-gate. The geometry of the side-gate allows tuning of the QD-lead tunnel coupling in a region of constant electron number with appropriate orbital state. Using the side-gate effect we study the competition between Kondo correlations and superconducting pairing on the QD, observing a decrease in the supercurrent when the Kondo temperature is reduced below the superconducting energy gap in qualitati…
Semiconductor/superconductor hybrids exhibit a range of phenomena that can be exploited for the study of novel physics and the development of new technologies. Understanding the origin the energy spectrum of such hybrids is therefore a crucial goal. Here, we study Josephson junctions defined by shadow epitaxy on InAsSb/Al nanowires. The devices exhibit gate-tunable supercurrents at low temperatures and multiple Andreev reflections (MARs) at finite voltage bias. Under microwave irradiation, photon assisted tunneling (PAT) of MARs produces characteristic oscillating sidebands at quantized energi…
We calculate the supercurrent through a Josephson junction consisting of a phase-coherent metal particle (quantum dot), weakly coupled to two superconductors. The classical motion in the quantum dot is assumed to be chaotic on time scales greater than the ergodic time $τ_{erg}$, which itself is much smaller than the mean dwell time $τ_{dwell}$. The excitation spectrum of the Josephson junction has a gap $E_{gap}$, which can be less than the gap $Δ$ in the bulk superconductors. The average supercurrent is computed in the ergodic regime $τ_{erg} \ll \hbar/Δ$, using random-matrix theory, and in t…
We present the results of theoretical study of Current-Phase Relations (CPR) in Josephson junctions of SIsFS type, where 'S' is a bulk superconductor and 'IsF' is a complex weak link consisting of a superconducting film 's', a metallic ferromagnet 'F' and an insulating barrier 'I'. We calculate the relationship between Josephson current and phase difference. At temperatures close to critical, calculations are performed analytically in the frame of the Ginsburg-Landau equations. At low temperatures numerical method is developed to solve selfconsistently the Usadel equations in the structure. We…
We show that the S/F/S Josephson $φ_0$-junction permits detection of macroscopic quantum tunneling and quantum oscillation of the magnetic moment by measuring the ac voltage across the junction. Exact expression for the tunnel splitting renormalized by the interaction with the superconducting order parameter is obtained. It is demonstrated that magnetic tunneling may become frozen at a sufficiently large $φ_0$. The quality factor of quantum oscillations of the magnetic moment due to finite Ohmic resistance of the junction is computed. It is shown that magnetic tunneling rate in the $φ_0$-junct…
The non-symmetrized current noise is crucial for the analysis of light emission in nanojunctions. The latter represent non-classical photon emitters whose description requires a full quantum approach. It was found experimentally that light emission can occur with a photon energy exceeding the applied dc voltage, which intuitively should be forbidden due to the Pauli principle. This overbias light emission cannot be described by the single-electron physics, but can be explained by two-electron or even three-electron processes, correlated by a local resonant mode in analogy to the well-known dyn…
We demonstrate that a suspended nanowire forming a weak link between two superconductors can be cooled to its motional ground state by a supercurrent flow. The predicted cooling mechanism has its origins in magnetic field induced inelastic tunneling of the macroscopic superconducting phase associated with the junction. Furthermore, we show the voltage-drop over the junction is proportional to the average population of the vibrational modes in the stationary regime, a phenomena which can be used to probe the level of cooling.
Carbon nanotubes (CNTs) are not intrinsically superconducting but they can carry a supercurrent when connected to superconducting electrodes. This supercurrent is mainly transmitted by discrete entangled electron-hole states confined to the nanotube, called Andreev Bound States (ABS). These states are a key concept in mesoscopic superconductivity as they provide a universal description of Josephson-like effects in quantum-coherent nanostructures (e.g. molecules, nanowires, magnetic or normal metallic layers) connected to superconducting leads. We report here the first tunneling spectroscopy of…
Josephson effect in short ballistic SINIS and SIFIS double-tunnel junctions, consisting of clean superconductors (S), a normal metal (N) or metallic ferromagnet (F), and insulating interfaces (I) is studied. For SINIS double-tunnel junctions, sharp peaks in the critical Josephson current as a function of the junction width result from the resonant amplification of the Andreev process when the quasi-bound states enter the superconducting gap. For SIFIS double-tunnel junctions spin split quasi-bound states partially amplify the supercurrent and trigger the transitions between 0 and $π$ states of…
We have observed that submicron sized Al--AlO{$_x$}--Al tunnel junctions can be stabilized completely by annealing them in vacuum at temperatures between $350^{\circ}$C and $450^{\circ}$C. In addition, low temperature characterization of the samples after the annealing treatment showed a marked improvement of the tunneling characteristics due to disappearance of unwanted resonances in the current. Charging energy, tunneling resistance, barrier thickness and height all increase after the treatment. The superconducting gap is not affected, but supercurrent is reduced in accordance with the incre…
We analyse the full counting statistics (FCS) of a superconducting junction in non-equilibrium in the limit of small interface transparency. In this limit we treat both supercurrent and multiple Andreev reflections on equal footing and show how to generalise previous results for both phenomena. Furthermore, we also allow for different gaps of both superconductors and investigate the intermediate regime which allows to make contact with previous results on normal-superconductor heterostructures. We also compare our predictions in this regime to experimental data.
We investigate ac Josephson effect in the resonant tunneling through mesoscopic superconducting junctions. In the presence of microwave irradiation, we show that the trajectory of multiple Andreev reflections can be closed by emitting or absorbing photons. Consequently, photon-assisted Andreev states are formed and play the role of carrying supercurrent. On the Shapiro steps, dc component appears when the resonant level is near a series of positions with spacing of half of the microwave frequency. Analytical result is derived in the limit of infinite superconducting gap, based on which new fea…
