We analyze recent experiments on the dilute rare-earth compound LiHo_xY_(1-x)F_4 in the context of an effective Ising dipolar model. Using a Monte Carlo method we calculate the low-temperature behavior of the specific heat and linear susceptibility, and compare our results to measurements. In our model the susceptibility follows a Curie-Weiss law at high temperature, chi ~ 1/(T-T_cw), with a Curie-Weiss temperature that scales with dilution, T_cw ~ x, consistent with early experiments. We also find that the peak in the specific heat scales linearly with dilution, C_max(T) ~ x, in disagreement with recent experiments. Experimental studies do not reach a consensus on the functional form of these quantities, and in particular we do not see reported scalings of the form chi ~ T^-0.75 and chi ~ exp(-T/T_0). Furthermore we calculate the ground state magnetization as a function of dilution, and re-examine the phase diagram around the critical dilution x_c=0.24(3). We find that the spin glass susceptibility for the Ising model does not diverge below x_c, while recent experiments give strong evidence for a stable spin-glass phase in LiHo_0.167Y_0.833F_4.
AC susceptibility measurements are presented on the dilute, dipolar coupled, Ising magnet LiHo$_x$Y$_{1-x}$F$_4$ for a concentration $x = 0.045$. The frequency and temperature dependences of the susceptibility show characteristic glassy relaxation. The absorption spectrum is found to broaden with decreasing temperature suggesting that the material is behaving as a spin glass and not as an exotic spin liquid as was previously observed. A dynamical scaling analysis suggests a spin glass transition temperature of 42.6 mK $\pm 2$ mK with an exponent $zν= 7.8 \pm 0.23$.
The physics of the spin glass (SG) state, with magnetic moments (spins) frozen in random orientations, is one of the most intriguing problems in condensed matter physics. While most theoretical studies have focused on the Edwards-Anderson model of Ising spins with only discrete `up/down' directions, such Ising systems are experimentally rare. LiHo$_{x}$Y$_{1-x}$F$_{4}$, where the Ho$^{3+}$ moments are well described by Ising spins, is an almost ideal Ising SG material. In LiHo$_{x}$Y$_{1-x}$F$_{4}$, the Ho$^{3+}$ moments interact predominantly via the inherently frustrated magnetostatic dipole…
We study the effective long-range Ising dipole model with a local exchange interaction appropriate for the dilute magnetic compound LiHo_{x}Y_{1-x}F_4. Our calculations yield a value of 0.12 K for the nearest neighbor exchange interaction. Using a Monte Carlo method we calculate the phase boundary T_c(x) between the ferromagnetic and paramagnetic phases. We demonstrate that the experimentally observed linear decrease in T_c with dilution is not the simple mean-field result, but a combination of the effects of fluctuations, the exchange interaction and the hyperfine coupling. Furthermore, we fi…
In LiHo_xY_{1-x}F4, the magnetic Holmium Ho^{3+} ions behave as effective Ising spins that can point parallel or antiparallel to the crystalline c-axis. The predominant inter-Holmium interaction is dipolar, while the Y^{3+} ions are non-magnetic. The application of a magnetic field Bx transverse to the c-axis Ising direction leads to quantum spin-flip fluctuations, making this material a rare physical realization of the celebrated transverse field Ising model. The problems of classical and transverse-field-induced quantum phase transitions in LiHo_xY_{1-x}F_4 in the dipolar ferromagnetic (x=1)…
Spin ice materials, such as Dy2Ti2O7 and Ho2Ti2O7, have been the subject of much interest for over the past fifteen years. Their low temperature strongly correlated state can be mapped onto the proton disordered state of common water ice and, consequently, spin ices display the same low temperature residual Pauling entropy as water ice. Interestingly, it was found in a previous study [X. Ke {\it et. al.} Phys. Rev. Lett. {\bf 99}, 137203 (2007)] that, upon dilution of the magnetic rare-earth ions (Dy^{3+} and Ho^{3+}) by non-magnetic Yttrium (Y^{3+}) ions, the residual entropy depends {\it non…
We simulate the dc magnetic response of the diluted dipolar-coupled Ising magnet LiHo\(_{0.045}\)Y\(_{0.955}\)F\(_4\) in a transverse field, using exact diagonalization of a two-spin Hamiltonian averaged over nearest-neighbour configurations. The pairwise model, incorporating hyperfine interactions, accounts for the observed drop-off in the longitudinal (c-axis) susceptibility with increasing transverse field; with the inclusion of a small tilt in the transverse field, it also accounts for the behavior of the off-diagonal magnetic susceptibility. The hyperfine interactions do not appear to lea…
We present analytical and numerical evidence for the validity of an effective S=1/2 approach to the description of random field generation in S>=1, and especially in an S=1, dipolar spin glass models with strong uniaxial Ising anisotropy and subject to weak external magnetic field Bx transverse to the Ising direction. Explicitely Bx-dependent random fields are shown to naturally emerge in the effective low-energy description of a microscopic S=1 toy model. We discuss our results in relation to recent theoretical studies pertaining to the topic of Bx-induced random fields in the LiHo$_x$Y$_{1-x…
By tempered Monte Carlo simulations, we study 2D site-diluted dipolar Ising systems. Dipoles are randomly placed on a fraction x of all L^2 sites in a square lattice, and point along a common crystalline axis. For x_c< x<=1, where x_c = 0.79(5), we find an antiferromagnetic phase below a temperature which vanishes as x approaches x_c from above. At lower values of x, we study (i) distributions of the spin--glass (SG) overlap q, (ii) their relative mean square deviation Delta_q^2 and kurtosis and (iii) xi_L/L, where xi_L is a SG correlation length. From their variation with temperature and syst…
Using Monte Carlo simulations, we study the character of the spin-glass (SG) state of a site-diluted dipolar Ising model. We consider systems of dipoles randomly placed on a fraction x of all L^3 sites of a simple cubic lattice that point up or down along a given crystalline axis. For x < 0.65 these systems are known to exhibit an equilibrium spin-glass phase below a temperature T_sg proportional to x. At high dilution and very low temperatures, well deep in the SG phase, we find spiky distributions of the overlap parameter q that are strongly sample-dependent. We focus on spikes associated wi…
By tempered Monte Carlo simulations, we study site-diluted Ising systems of magnetic dipoles. All dipoles are randomly placed on a fraction x of all L^3 sites of a simple cubic lattice, and point along a given crystalline axis. For x_c< x<=1, where x_c = 0.65, we find an antiferromagnetic phase below a temperature which vanishes as x tends to x_c from above. At lower values of x, we find an equilibrium spin-glass (SG) phase below a temperature given by k_B T_{sg} = x e_d, where e_d is a nearest neighbor dipole-dipole interaction energy. We study (a) the relative mean square deviation D_q^2 of …
We study the pair correlation of Active Brownian Particles at low density using numerical simulations and analytical calculations. We observe a winged pair correlation: while particles accumulate in front of an active particle as expected, the depletion wake consists of two depletion wings. In the limit of soft particles, we obtain a closed equation for the pair correlation, allowing us to characterize the depletion wings. In particular, we unveil two regimes at high activity where the wings adopt a self-similar profile and decay algebraically. We also perform experiments of self-propelled Jan…
Dilute dipolar Ising magnets remain a notoriously hard problem to tackle both analytically and numerically because of long-ranged interactions between spins as well as rare region effects. We study a new type of anisotropic dilute dipolar Ising system in three dimensions [Phys. Rev. Lett. {\bf 114}, 247207 (2015)] that arises as an effective description of randomly diluted classical spin ice, a prototypical spin liquid in the disorder-free limit, with a small fraction $x$ of non-magnetic impurities. Metropolis algorithm within a parallel thermal tempering scheme fails to achieve equilibration …
Dilute dipolar systems in three dimensions are expected to undergo a spin glass transition as the temperature decreases. Contrary to this, we find from Wang-Landau Monte Carlo simulations that at low concentrations $x$, dipoles randomly placed on a cubic lattice with dipolar interactions do not undergo a phase transition. We find that in the thermodynamic limit the ``glass'' transition temperature $T_g$ goes to zero as $1/\sqrt{N}$ where $N$ is the number of dipoles. The entropy per particle at low temperatures is larger for lower concentrations ($x=4.5%$) than for higher concentrations ($x=20…
The LiHo$_x$Y$_{1-x}$F$_4$ Ising magnetic material subject to a magnetic field, $B_x$, perpendicular to the Ho$^{3+}$ Ising direction has shown over the past twenty years to be a host of very interesting thermodynamic and magnetic phenomena. Unfortunately, the availability of other magnetic materials other than LiHo$_x$Y$_{1-x}$F$_4$ that may be described by a transverse field Ising model remains very much limited. It is in this context that we use here mean-field theory to investigate the suitability of the Ho(OH)$_{3}$, Dy(OH)$_{3}$ and Tb(OH)$_3$ insulating hexagonal dipolar Ising-like ferr…
We study the temperature-dilution phase diagram of a site-diluted Heisenberg antiferromagnet on a fcc lattice, with and without the Dzyaloshinskii-Moriya anisotropic term, fixed to realistic microscopic parameters for $IIB_{1-x} Mn_x Te$ (IIB=Cd, Hg, Zn). We show that the dipolar Dzyaloshinskii-Moriya anisotropy induces a finite-temperature phase transition to a spin glass phase, at dilutions larger than 80%. The resulting probability distribution of the order parameter P(q) is similar to the one found in the cubic lattice Edwards-Anderson Ising model. The critical exponents undergo large fini…
We study a Bose-Einstein condensate (BEC) of a dilute gas with dipolar interactions, at finite temperature, using the Hartree-Fock-Bogoliubov (HFB) theory within the Popov approximation. An additional approximation involving the dipolar exchange interaction is made to facilitate the computation. We calculate the temperature dependence of the condensate fraction of a condensate confined in a cylindrically symmetric harmonic trap. We show that the bi-concave shaped condensates found in Ref. \cite{Ronen07} in certain pancake traps at zero temperature, are also stable at finite temperature. Surpri…
We consider a dilute gas of dipole moments in an arbitrary harmonic trap and treat both the short-range, isotropic delta-interaction and the long-range, anisotropic dipole-dipole interaction perturbatively. With this we calculate the leading shift of the critical temperature with respect to that of an ideal gas as a function of the relative orientation of the dipole moments with respect to the harmonic trap axes. In particular, we determine those magic angles, where the dipolar shift of the Bose-Einstein condensation temperature vanishes. Furthermore, we show for the parameters of the ongoing …
Experimental data of the frequency-dependent ac susceptibility for the dipolar spin ice Dy2Ti2O7 has been analyzed by Monte Carlo simulations on the basis of the single-spin-flip Metropolis algorithm. We have directly evaluated the ac susceptibility by applying an ac magnetic field. We found that the simulated behaviors reproduces the experimental behavior of the ac susceptibility in the temperature range from 0.6 to 1.0 K, where dilute magnetic monopoles diffusively move. The conversion factor from simulation time to real time, i.e., the rate of hopping of monopoles to nearest-neighbor sites,…
The low-density expansions for the energy, chemical potential, and condensate depletion of the homogeneous dilute dipolar Bose gas are obtained by regularizing the dipole-dipole interaction at long distances. It is shown that the leading term, proportional to the density, allows a simple physical interpretation and consistently describes the thermodynamic stability of the system. The long-range asymptotics are obtained analytically for the normal and anomalous one-particle correlation functions and the pair distribution function. We discuss the properties of the two-body scattering with zero r…
The nonlinear magnetic $χ_{3}$ and spin-glass $χ_{sg}$ susceptibilities in zero applied field are obtained, from tempered Monte Carlo simulations, for three different spin glasses (SGs) of Ising spins with quenched site disorder. We find that the relation $-T^3χ_3=χ_{sg}-2/3$ ($T$ is the temperature), which holds for Edwards-Anderson SGs, is approximately fulfilled in canonical-like SGs. For nearest neighbor antiferromagnetic interactions, on a 0.4 fraction of all sites in fcc lattices, as well as for spatially disordered Ising dipolar (DID) systems, $-T^3χ_3$ and $χ_{sg}$ appear to diverge in…
The static dielectric properties of dense ionic fluids, e.g., room temperature ionic liquids (RTILs) and inorganic fused salts, are investigated on different length scales by means of grandcanonical Monte Carlo simulations. A generally applicable scheme is developed which allows one to approximately decompose the electric susceptibility of dense ionic fluids into the orientation and the distortion polarization contribution. It is shown that at long range the well-known plasma-like perfect screening behavior occurs, which corresponds to a diverging distortion susceptibility, whereas at short ra…
Using tempered Monte Carlo simulations, we study the the spin-glass phase of dense packings of Ising dipoles pointing along random axes. We consider systems of L^3 dipoles (a) placed on the sites of a simple cubic lattice with lattice constant $d$, (b) placed at the center of randomly closed packed spheres of diameter d that occupy a 64% of the volume. For both cases we find an equilibrium spin-glass phase below a temperature T_sg. We compute the spin-glass overlap parameter q and their associated correlation length xi_L. From the variation of xi_L with T and L we determine T_sg for both syste…
