An analysis of the optical response of periodically arrayed monolayers composed of dielectric spheres with low refractive index is herein presented. The reflectance spectra of two-dimensional square and triangular lattices are obtained by means of the vector Korringa-Kohn-Rostoker method, both spectra showing very similar qualitative features for photon energies below the onset of diffraction spots. In this energy region, the same number of peaks of unitary amplitude in the reflectance spectra are predicted for both kinds of monolayers, suggesting that this must be a universal feature independent of the particular geometry of the lattice. The origin of these high reflectance peaks is investigated. It is found that the resonances of TM and TE modes due to dipolar, quadrupolar and octupolar interaction inside the monolayer are largely responsible for the peak structure observed in the reflectance spectra.
In this work, a refractive index (RI) sensor with an effective integration of colorimetric detection and optical sensing capabilities has been developed. Colorimetric detection relies on the sensitivity of the structural color of photonic crystal (PC) substrates to the changes in background RI, while the optical sensing is performed by measuring the magnification abilities of the dielectric microspheres, which depends on the position of the photonic nanojet. Based on this concept, we have successfully assembled 35 μm-diameter barium titanate glass microspheres, 4.9 μm-diameter polystyrene and …
We report strong coupling of a monolayer of J-aggregated dye molecules to the whispering gallery modes of a dielectric microsphere at room temperature. We systematically studied the evolution of strong coupling as the number of layers of dye molecules was increased, we found the Rabi splitting to rise from 56 meV for a single layer to 94 meV for four layers of dye molecules. We compare our experimental results with 2D numerical simulations and a simple coupled oscillator model, finding good agreement. We anticipate that these results will act as a stepping stone for integrating molecule-cavity…
Forces and torques exerted on dielectric disks trapped in a Gaussian standing wave are analyzed theoretically for disks of radius $2~μ\text{m}$ with index of refraction $n=1.45$ and $n=2.0$ as well as disks of radius 200 nm with $n=1.45$. Calculations of the forces and torques were conducted both analytically and numerically using a discrete-dipole approximation method. Besides harmonic terms, third order ro-translational coupling terms in the potential energy can be significant and a necessary consideration when describing the dynamics of disks outside of the Rayleigh limit. The coupling term…
The manipulation of light emitted by two-dimensional semiconductors grounds forthcoming technologies in the field of on-chip communications. However, these technologies require from the so elusive out-of-plane photon sources to achieve an efficient coupling of radiated light into planar devices. Here we propose a versatile spectroscopic method that enables the identification of the out-of-plane component of dipoles. The method is based on the selective coupling of light emitted by in-plane and out-of-plane dipoles to the whispering gallery modes of spherical dielectric microresonators, in clos…
Treatment of Linear and Nonlinear Dielectric Property of Molecular Monolayer and Submonolayer with Microscopic Dipole Lattice Model: I. Second Harmonic Generation and Sum-Frequency Generation
Strong enhancement of molecular circular dichroism has the potential to enable efficient asymmetric photolysis, a method of chiral separation that has conventionally been impeded by insufficient yield and low enantiomeric excess. Here, we study experimentally how predicted enhancements in optical chirality density near resonant silicon nanodisks boost circular dichroism. We use fluorescence-detected circular dichroism spectroscopy to measure indirectly the differential absorption of circularly polarized light by a monolayer of optically active molecules functionalized to silicon nanodisk array…
We develop the theory of transportation and localization of a transparent dielectric spherical particle with the gradient forces in the interference field of orthogonally directed standing laser waves $E_z (\cos kz)$ and $E_x (\cos kx)$. It is shown that, when the waves $E_z$ and $E_x$ are coherent, the interference radiation field contains two harmonic components with the periods $Λ_0=π/k$ and $Λ_Δ=π/(k \sin (π/4))$. The amplitudes of the gradient force components depend on the ratio of the particle radius $R$ to the modulation periods due to inhomogeneity of radiation in the particle volume …
Here we propose a method of the excitation of perpendicular standing spin waves (PSSWs) of different orders in an optomagnonic microcavity by ultrashort laser pulses. The microcavity is formed by a magnetic dielectric film surrounded by dielectric non-magnetic Bragg mirrors. Optical cavity modes in the magnetic layer provide concentration and strongly non-uniform distribution of the optical power over the layer thickness and therefore induce the effective field of the inverse Faraday effect also spatially non-uniform. It results in excitation of PSSWs. PSSWs whose wavevector is closest to the …
Due to their high circulating intensities, ultra-high quality factor dielectric whispering-gallery mode resonators have enabled the development of low threshold Raman microlasers. Subsequently, other Raman-related phenomena, such as cascaded stimulated Raman scattering (CSRS) and stimulated anti-Stokes Raman scattering (SARS), were observed. While low threshold frequency conversion and generation have clear applications, CSRS and SARS have been limited by the low Raman gain. In this work, the surface of a silica resonator is modified with an organic monolayer, increasing the Raman gain. Up to …
Systems with strong light-matter interaction opens up new avenues for studying topological phases of matter. Examples include exciton-polaritons, mixed light-matter quasiparticles, where the topology of the polaritonic band structure arises from the collective coupling between matter wave and optical fields strongly confined in periodic dielectric structures. Distinct from light-matter interaction in a uniform environment, the spatially varying nature of the optical fields leads to a fundamental modification of the well-known optical selection rules, which were derived under the plane wave app…
Effective refractive index of disordered all-dielectric metasurfaces consisting of gallium phosphide (GaP) spheres is studied by means of three-dimensional finite-difference time-domain (FDTD) simulations at the wavelength of 532~nm. It is shown that a mixture of the high index nanoparticles with sizes close to the first magnetic and electric resonances randomly dispersed on metasurface may possess negative refraction. The dependence of the metasurface effective refractive index on the nanoparticle concentration and size is constructed. The feasibility of negative refraction at large concentra…
