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arXiv 0712.3577physics.atom-phphysics.optics
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从稀有气体原子高次谐波谱中提取与物种有关的偶极矩

Extraction of the species dependent dipole moment from high-order harmonic spectra in rare gas atoms

Anh-Thu Le, Toru Morishita, C. D. Lin

摘要:

基于求解含时薛定谔方程得到的原子高次谐波产生谱,定量地建立了高次谐波产额可以表示为返回电子波包与光复合截面的乘积,且返回波包的形状与原子种类无关.通过比较不同靶在相同激光脉冲下产生的高次谐波谱,可以得到精确的结构信息,包括复合振幅的相位。这一结果为从短脉冲激光产生的高次谐波谱研究复杂系统的目标结构,包括它们的时间演化提供了可能性。

英文摘要:

Based on high-order harmonic generation (HHG) spectra obtained from solving the time-dependent Schrodinger equation for atoms, we established quantitatively that the HHG yield can be expressed as the product of a returning electron wave packet and the photo-recombination cross sections, and the shape of the returning wave packet is shown to be largely independent of the species. By comparing the HHG spectra generated from different targets under identical laser pulses, accurate structural information, including the phase of the recombination amplitude, can be retrieved. This result opens up the possibility of studying the target structure of complex systems, including their time evolution, from the HHG spectra generated by short laser pulses.

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